Abstract：
:Over the history of carbon, it is generally acknowledged that Bernal AB stacking of the sp2 carbon layers is the unique crystalline form of graphite. The universal graphite structure is synthesized at 2,600~3,000 °C and exhibits a micro-polycrystalline feature. In this paper, we provide evidence for a metastable form of graphite with an AA' structure. The non-Bernal AA' allotrope of graphite is synthesized by the thermal- and plasma-treatment of graphene nanopowders at ~1,500 °C. The formation of AA' bilayer graphene nuclei facilitates the preferred texture growth and results in single-crystal AA' graphite in the form of nanoribbons (1D) or microplates (2D) of a few nm in thickness. Kinetically controlled AA' graphite exhibits unique nano- and single-crystalline feature and shows quasi-linear behavior near the K-point of the electronic band structure resulting in anomalous optical and acoustic phonon behavior.
journal_name
Sci Repjournal_title
Scientific reportsauthors
Lee JK,Kim JG,Hembram KP,Kim YI,Min BK,Park Y,Lee JK,Moon DJ,Lee W,Lee SG,John Pdoi
10.1038/srep39624subject
Has Abstractpub_date
2016-12-21 00:00:00pages
39624issn
2045-2322pii
srep39624journal_volume
6pub_type
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