Abstract:
:Building porosity in monolithic materials is highly desired to design 3D electrodes, however ex-situ introduction or in-situ generation of nano-scale sacrificial template is still a great challenge. Here Al-Si eutectic droplet templates are uniformly injected into bulk Si through Al-induced solid-solid convection to construct a highly porous Si framework. This process is concomitant with process-inherent conformal coating of ion-conductive oxide. Such an all-in-one method has generated a (continuously processed) high-capacity Si anode integrating longevity and stable electrolyte-anode diaphragm for Li-ion batteries (e.g. a reversible capacity as large as ~1800 mAh/g or ~350 μAh/cm(2)-μm with a CE of ~99% at 0.1 C after long-term 400 cycles).
journal_name
Sci Repjournal_title
Scientific reportsauthors
Qu F,Li C,Wang Z,Wen Y,Richter G,Strunk HPdoi
10.1038/srep10381subject
Has Abstractpub_date
2015-05-19 00:00:00pages
10381issn
2045-2322pii
srep10381journal_volume
5pub_type
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