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Abnormal phase transition between two-dimensional high-density liquid crystal and low-density crystalline solid phases.

Abstract：

:Some two-dimensional liquid systems are theoretically predicted to have an anomalous phase transition due to unique intermolecular interactions, for example the first-order transition between two-dimensional high-density water and low-density amorphous ice. However, it has never been experimentally observed, to the best of our knowledge. Here we report an entropy-driven phase transition between a high-density liquid crystal and low-density crystalline solid, directly observed by scanning tunneling microscope in carbon monoxide adsorbed on Cu(111). Combined with first principle calculations, we find that repulsive dipole-dipole interactions between carbon monoxide molecules lead to unconventional thermodynamics. This finding of unconventional thermodynamics in two-dimensional carbon monoxide not only provides a platform to study the fundamental principles of anomalous phase transitions in two-dimensional liquids at the atomic scale, but may also help to design and develop more efficient copper-based catalysis.

journal_name

Nat Commun

journal_title

Nature communications

authors

Li W,Kong L,Feng B,Fu H,Li H,Zeng XC,Wu K,Chen L

doi

10.1038/s41467-017-02634-6

subject

Has Abstract

pub_date

2018-01-15 00:00:00

pages

198

issue

1

issn

2041-1723

pii

10.1038/s41467-017-02634-6

journal_volume

9

pub_type

杂志文章

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