Unusual behavior of cuprates explained by heterogeneous charge localization.

Abstract:

:The discovery of high-temperature superconductivity in cuprates ranks among the major scientific milestones of the past half century, yet pivotal questions regarding the complex phase diagram of these materials remain unanswered. Generally thought of as doped charge-transfer insulators, these complex oxides exhibit pseudogap, strange-metal, superconducting, and Fermi liquid behavior with increasing hole-dopant concentration. Motivated by recent experimental observations, here we introduce a phenomenological model wherein exactly one hole per planar copper-oxygen unit is delocalized with increasing doping and temperature. The model is percolative in nature, with parameters that are highly consistent with experiments. It comprehensively captures key unconventional experimental results, including the temperature and the doping dependence of the pseudogap phenomenon, the strange-metal linear temperature dependence of the planar resistivity, and the doping dependence of the superfluid density. The success and simplicity of the model greatly demystify the cuprate phase diagram and point to a local superconducting pairing mechanism.

journal_name

Sci Adv

journal_title

Science advances

authors

Pelc D,Popčević P,Požek M,Greven M,Barišić N

doi

10.1126/sciadv.aau4538

subject

Has Abstract

pub_date

2019-01-25 00:00:00

pages

eaau4538

issue

1

issn

2375-2548

pii

aau4538

journal_volume

5

pub_type

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