Efficient table-top dual-wavelength beamline for ultrafast transient absorption spectroscopy in the soft X-ray region.

Abstract:

:We present a table-top beamline providing a soft X-ray supercontinuum extending up to 370 eV from high-order harmonic generation with sub-13 fs 1300 nm driving pulses and simultaneous production of sub-5 fs pulses centered at 800 nm. Optimization of high harmonic generation in a long and dense gas medium yields a photon flux of  ~ 1.4 × 106 photons/s/1% bandwidth at 300 eV. The temporal resolution of X-ray transient absorption experiments with this beamline is measured to be 11 fs for 800 nm excitation. This dual-wavelength approach, combined with high flux and high spectral and temporal resolution soft X-ray absorption spectroscopy, is a new route to the study of ultrafast electronic dynamics in carbon-containing molecules and materials at the carbon K-edge.

journal_name

Sci Rep

journal_title

Scientific reports

authors

Barreau L,Ross AD,Garg S,Kraus PM,Neumark DM,Leone SR

doi

10.1038/s41598-020-62461-6

subject

Has Abstract

pub_date

2020-04-01 00:00:00

pages

5773

issue

1

issn

2045-2322

pii

10.1038/s41598-020-62461-6

journal_volume

10

pub_type

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