Energy-temperature uncertainty relation in quantum thermodynamics.

Abstract:

:It is known that temperature estimates of macroscopic systems in equilibrium are most precise when their energy fluctuations are large. However, for nanoscale systems deviations from standard thermodynamics arise due to their interactions with the environment. Here we include such interactions and, using quantum estimation theory, derive a generalised thermodynamic uncertainty relation valid for classical and quantum systems at all coupling strengths. We show that the non-commutativity between the system's state and its effective energy operator gives rise to quantum fluctuations that increase the temperature uncertainty. Surprisingly, these additional fluctuations are described by the average Wigner-Yanase-Dyson skew information. We demonstrate that the temperature's signal-to-noise ratio is constrained by the heat capacity plus a dissipative term arising from the non-negligible interactions. These findings shed light on the interplay between classical and non-classical fluctuations in quantum thermodynamics and will inform the design of optimal nanoscale thermometers.

journal_name

Nat Commun

journal_title

Nature communications

authors

Miller HJD,Anders J

doi

10.1038/s41467-018-04536-7

subject

Has Abstract

pub_date

2018-06-06 00:00:00

pages

2203

issue

1

issn

2041-1723

pii

10.1038/s41467-018-04536-7

journal_volume

9

pub_type

杂志文章
  • Immunoregulation of macrophages by dynamic ligand presentation via ligand-cation coordination.

    abstract::Macrophages regulate host responses to implants through their dynamic adhesion, release, and activation. Herein, we employ bisphosphonate (BP)-coated gold nanoparticle template (BNP) to direct the swift and convertible formation of Mg2+-functional Mg2+-BP nanoparticle (NP) on the BP-AuNP surface via reversible Mg2+-BP...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-09733-6

    authors: Kang H,Yang B,Zhang K,Pan Q,Yuan W,Li G,Bian L

    更新日期:2019-04-12 00:00:00

  • Dense and accurate whole-chromosome haplotyping of individual genomes.

    abstract::The diploid nature of the human genome is neglected in many analyses done today, where a genome is perceived as a set of unphased variants with respect to a reference genome. This lack of haplotype-level analyses can be explained by a lack of methods that can produce dense and accurate chromosome-length haplotypes at ...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-017-01389-4

    authors: Porubsky D,Garg S,Sanders AD,Korbel JO,Guryev V,Lansdorp PM,Marschall T

    更新日期:2017-11-03 00:00:00

  • Gelation process visualized by aggregation-induced emission fluorogens.

    abstract::Alkaline-urea aqueous solvent system provides a novel and important approach for the utilization of polysaccharide. As one of the most important polysaccharide, chitosan can be well dissolved in this solvent system, and the resultant hydrogel material possesses unique and excellent properties. Thus the sound understan...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms12033

    authors: Wang Z,Nie J,Qin W,Hu Q,Tang BZ

    更新日期:2016-06-23 00:00:00

  • Mechanically interlocked functionalization of monoclonal antibodies.

    abstract::Because monoclonal antibodies (mAbs) have exceptional specificity and favorable pharmacology, substantial efforts have been made to functionalize them, either with potent cytotoxins, biologics, radionuclides, or fluorescent groups for therapeutic benefit and/or use as theranostic agents. To exploit our recently discov...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-03976-5

    authors: Bzymek KP,Puckett JW,Zer C,Xie J,Ma Y,King JD,Goodstein LH,Avery KN,Colcher D,Singh G,Horne DA,Williams JC

    更新日期:2018-04-20 00:00:00

  • Using controlled disorder to probe the interplay between charge order and superconductivity in NbSe2.

    abstract::The interplay between superconductivity and charge-density wave (CDW) in 2H-NbSe2 is not fully understood despite decades of study. Artificially introduced disorder can tip the delicate balance between two competing long-range orders, and reveal the underlying interactions that give rise to them. Here we introduce dis...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-05153-0

    authors: Cho K,Kończykowski M,Teknowijoyo S,Tanatar MA,Guss J,Gartin PB,Wilde JM,Kreyssig A,McQueeney RJ,Goldman AI,Mishra V,Hirschfeld PJ,Prozorov R

    更新日期:2018-07-18 00:00:00

  • Scaling law for excitons in 2D perovskite quantum wells.

    abstract::Ruddlesden-Popper halide perovskites are 2D solution-processed quantum wells with a general formula A2A'n-1M n X3n+1, where optoelectronic properties can be tuned by varying the perovskite layer thickness (n-value), and have recently emerged as efficient semiconductors with technologically relevant stability. However,...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-04659-x

    authors: Blancon JC,Stier AV,Tsai H,Nie W,Stoumpos CC,Traoré B,Pedesseau L,Kepenekian M,Katsutani F,Noe GT,Kono J,Tretiak S,Crooker SA,Katan C,Kanatzidis MG,Crochet JJ,Even J,Mohite AD

    更新日期:2018-06-08 00:00:00

  • The increasing likelihood of temperatures above 30 to 40 °C in the United Kingdom.

    abstract::As European heatwaves become more severe, summers in the United Kingdom (UK) are also getting warmer. The UK record temperature of 38.7 °C set in Cambridge in July 2019 prompts the question of whether exceeding 40 °C is now within reach. Here, we show how human influence is increasing the likelihood of exceeding 30, 3...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-16834-0

    authors: Christidis N,McCarthy M,Stott PA

    更新日期:2020-06-30 00:00:00

  • Multiplexed imaging of nucleome architectures in single cells of mammalian tissue.

    abstract::The three-dimensional architecture of the genome affects genomic functions. Multiple genome architectures at different length scales, including chromatin loops, domains, compartments, and lamina- and nucleolus-associated regions, have been discovered. However, how these structures are arranged in the same cell and how...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-16732-5

    authors: Liu M,Lu Y,Yang B,Chen Y,Radda JSD,Hu M,Katz SG,Wang S

    更新日期:2020-06-09 00:00:00

  • Two distinct catalytic pathways for GH43 xylanolytic enzymes unveiled by X-ray and QM/MM simulations.

    abstract::Xylanolytic enzymes from glycoside hydrolase family 43 (GH43) are involved in the breakdown of hemicellulose, the second most abundant carbohydrate in plants. Here, we kinetically and mechanistically describe the non-reducing-end xylose-releasing exo-oligoxylanase activity and report the crystal structure of a native ...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-20620-3

    authors: Morais MAB,Coines J,Domingues MN,Pirolla RAS,Tonoli CCC,Santos CR,Correa JBL,Gozzo FC,Rovira C,Murakami MT

    更新日期:2021-01-14 00:00:00

  • An unusual endo-selective C-H hydroarylationof norbornene by the Rh(I)-catalyzed reactionof benzamides.

    abstract::Hydroarylation is an environmentally attractive strategy which incorporates all of the atoms contained in the substrates into the desired products. Almost all the hydroarylations of norbornene reported to date involve an exo-selective reaction. Here we show the endo-selective hydroarylation of norbornene in the Rh(I)-...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-017-01531-2

    authors: Shibata K,Natsui S,Tobisu M,Fukumoto Y,Chatani N

    更新日期:2017-11-13 00:00:00

  • Gas-responsive porous magnet distinguishes the electron spin of molecular oxygen.

    abstract::Gas-sensing materials are becoming increasingly important in our society, requiring high sensitivity to differentiate similar gases like N2 and O2. For the design of such materials, the driving force of electronic host-guest interaction or host-framework changes during the sorption process has commonly been considered...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-07889-1

    authors: Kosaka W,Liu Z,Zhang J,Sato Y,Hori A,Matsuda R,Kitagawa S,Miyasaka H

    更新日期:2018-12-21 00:00:00

  • Manipulating dehydrogenation kinetics through dual-doping Co3N electrode enables highly efficient hydrazine oxidation assisting self-powered H2 production.

    abstract::Replacing sluggish oxygen evolution reaction (OER) with hydrazine oxidation reaction (HzOR) to produce hydrogen has been considered as a more energy-efficient strategy than water splitting. However, the relatively high cell voltage in two-electrode system and the required external electric power hinder its scalable ap...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-15563-8

    authors: Liu Y,Zhang J,Li Y,Qian Q,Li Z,Zhu Y,Zhang G

    更新日期:2020-04-15 00:00:00

  • Cellobiohydrolase 1 from Trichoderma reesei degrades cellulose in single cellobiose steps.

    abstract::Cellobiohydrolase 1 from Trichoderma reesei (TrCel7A) processively hydrolyses cellulose into cellobiose. Although enzymatic techniques have been established as promising tools in biofuel production, a clear understanding of the motor's mechanistic action has yet to be revealed. Here, we develop an optical tweezers-bas...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms10149

    authors: Brady SK,Sreelatha S,Feng Y,Chundawat SP,Lang MJ

    更新日期:2015-12-10 00:00:00

  • Co-evolution of primitive methane-cycling ecosystems and early Earth's atmosphere and climate.

    abstract::The history of the Earth has been marked by major ecological transitions, driven by metabolic innovation, that radically reshaped the composition of the oceans and atmosphere. The nature and magnitude of the earliest transitions, hundreds of million years before photosynthesis evolved, remain poorly understood. Using ...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-16374-7

    authors: Sauterey B,Charnay B,Affholder A,Mazevet S,Ferrière R

    更新日期:2020-06-01 00:00:00

  • Continuous crystalline graphene papers with gigapascal strength by intercalation modulated plasticization.

    abstract::Graphene has an extremely high in-plane strength yet considerable out-of-plane softness. High crystalline order of graphene assemblies is desired to utilize their in-plane properties, however, challenged by the easy formation of chaotic wrinkles for the intrinsic softness. Here, we find an intercalation modulated plas...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-16494-0

    authors: Li P,Yang M,Liu Y,Qin H,Liu J,Xu Z,Liu Y,Meng F,Lin J,Wang F,Gao C

    更新日期:2020-05-27 00:00:00

  • Author Correction: The rapid electrochemical activation of MoTe2 for the hydrogen evolution reaction.

    abstract::An amendment to this paper has been published and can be accessed via a link at the top of the paper. ...

    journal_title:Nature communications

    pub_type: 已发布勘误

    doi:10.1038/s41467-019-13337-5

    authors: McGlynn JC,Dankwort T,Kienle L,Bandeira NAG,Fraser JP,Gibson EK,Cascallana-Matías I,Kamarás K,Symes MD,Miras HN,Ganin AY

    更新日期:2019-11-20 00:00:00

  • A novel mechanism of generating extracellular vesicles during apoptosis via a beads-on-a-string membrane structure.

    abstract::Disassembly of apoptotic cells into smaller fragments (a form of extracellular vesicle called apoptotic bodies) can facilitate removal of apoptotic debris and intercellular communication. However, the mechanism underpinning this process is unclear. While observing monocytes undergoing apoptosis by time-lapse microscop...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms8439

    authors: Atkin-Smith GK,Tixeira R,Paone S,Mathivanan S,Collins C,Liem M,Goodall KJ,Ravichandran KS,Hulett MD,Poon IK

    更新日期:2015-06-15 00:00:00

  • Heterologous biosynthesis and characterization of a glycocin from a thermophilic bacterium.

    abstract::The genome of the thermophilic bacterium, Aeribacillus pallidus 8, encodes the bacteriocin pallidocin. It belongs to the small class of glycocins and is posttranslationally modified, containing an S-linked glucose on a specific Cys residue. In this study, the pallidocin biosynthetic machinery is cloned and expressed i...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-09065-5

    authors: Kaunietis A,Buivydas A,Čitavičius DJ,Kuipers OP

    更新日期:2019-03-07 00:00:00

  • A microfluidic platform enabling single-cell RNA-seq of multigenerational lineages.

    abstract::We introduce a microfluidic platform that enables off-chip single-cell RNA-seq after multi-generational lineage tracking under controlled culture conditions. We use this platform to generate whole-transcriptome profiles of primary, activated murine CD8+ T-cell and lymphocytic leukemia cell line lineages. Here we repor...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms10220

    authors: Kimmerling RJ,Lee Szeto G,Li JW,Genshaft AS,Kazer SW,Payer KR,de Riba Borrajo J,Blainey PC,Irvine DJ,Shalek AK,Manalis SR

    更新日期:2016-01-06 00:00:00

  • Closing the gap between palaeontological and neontological speciation and extinction rate estimates.

    abstract::Measuring the pace at which speciation and extinction occur is fundamental to understanding the origin and evolution of biodiversity. Both the fossil record and molecular phylogenies of living species can provide independent estimates of speciation and extinction rates, but often produce strikingly divergent results. ...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-07622-y

    authors: Silvestro D,Warnock RCM,Gavryushkina A,Stadler T

    更新日期:2018-12-07 00:00:00

  • Boosting the catalysis of gold by O2 activation at Au-SiO2 interface.

    abstract::Supported gold (Au) nanocatalysts have attracted extensive interests in the past decades because of their unique catalytic properties for a number of key chemical reactions, especially in (selective) oxidations. The activation of O2 on Au nanocatalysts is crucial and remains a challenge because only small Au nanoparti...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-14241-8

    authors: Zhang Y,Zhang J,Zhang B,Si R,Han B,Hong F,Niu Y,Sun L,Li L,Qiao B,Sun K,Huang J,Haruta M

    更新日期:2020-01-28 00:00:00

  • Author Correction: Hypervirulent Listeria monocytogenes clones' adaptation to mammalian gut accounts for their association with dairy products.

    abstract::An amendment to this paper has been published and can be accessed via a link at the top of the paper. ...

    journal_title:Nature communications

    pub_type: 已发布勘误

    doi:10.1038/s41467-019-11625-8

    authors: Maury MM,Bracq-Dieye H,Huang L,Vales G,Lavina M,Thouvenot P,Disson O,Leclercq A,Brisse S,Lecuit M

    更新日期:2019-08-06 00:00:00

  • Publisher Correction: JMJD5 is a human arginyl C-3 hydroxylase.

    abstract::The originally published version of this Article contained an error in the spelling of the author Md. Saiful Islam, which was incorrectly given as Saiful Islam. This has now been corrected in both the PDF and HTML versions of the Article. ...

    journal_title:Nature communications

    pub_type: 杂志文章,已发布勘误

    doi:10.1038/s41467-018-04196-7

    authors: Wilkins SE,Islam MS,Gannon JM,Markolovic S,Hopkinson RJ,Ge W,Schofield CJ,Chowdhury R

    更新日期:2018-04-23 00:00:00

  • Publisher Correction: Stateful characterization of resistive switching TiO2 with electron beam induced currents.

    abstract::The original version of this Article contained an error in Eq. 1. The arrows between the symbols "T" and "B", and "B" and "T", were written "↔" but should have been "→", and incorrectly read: IEBIC=IEBAC+ISEE+I(e↔h)+IEBICT↔B+IESEEB↔T The correct from of the Eq. 1 is as follows:IEBIC=IEBAC+ISEE+I(e↔h)+IEBICT→B+IESEEB→T...

    journal_title:Nature communications

    pub_type: 杂志文章,已发布勘误

    doi:10.1038/s41467-018-02844-6

    authors: Hoskins BD,Adam GC,Strelcov E,Zhitenev N,Kolmakov A,Strukov DB,McClelland JJ

    更新日期:2018-01-24 00:00:00

  • Microscopic mechanism of biphasic interface relaxation in lithium iron phosphate after delithiation.

    abstract::Charge/discharge of lithium-ion battery cathode material LiFePO4 is mediated by the structure and properties of the interface between delithiated and lithiated phases. Direct observations of the interface in a partially delithiated single crystal as a function of time using scanning transmission electron microscopy an...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-05241-1

    authors: Kobayashi S,Kuwabara A,Fisher CAJ,Ukyo Y,Ikuhara Y

    更新日期:2018-07-20 00:00:00

  • Life cycle assessment needs predictive spatial modelling for biodiversity and ecosystem services.

    abstract::International corporations in an increasingly globalized economy exert a major influence on the planet's land use and resources through their product design and material sourcing decisions. Many companies use life cycle assessment (LCA) to evaluate their sustainability, yet commonly-used LCA methodologies lack the spa...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms15065

    authors: Chaplin-Kramer R,Sim S,Hamel P,Bryant B,Noe R,Mueller C,Rigarlsford G,Kulak M,Kowal V,Sharp R,Clavreul J,Price E,Polasky S,Ruckelshaus M,Daily G

    更新日期:2017-04-21 00:00:00

  • Plasmepsin II-III copy number accounts for bimodal piperaquine resistance among Cambodian Plasmodium falciparum.

    abstract::Multidrug resistant Plasmodium falciparum in Southeast Asia endangers regional malaria elimination and threatens to spread to other malaria endemic areas. Understanding mechanisms of piperaquine (PPQ) resistance is crucial for tracking its emergence and spread, and to develop effective strategies for overcoming it. He...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-04104-z

    authors: Bopp S,Magistrado P,Wong W,Schaffner SF,Mukherjee A,Lim P,Dhorda M,Amaratunga C,Woodrow CJ,Ashley EA,White NJ,Dondorp AM,Fairhurst RM,Ariey F,Menard D,Wirth DF,Volkman SK

    更新日期:2018-05-02 00:00:00

  • Controlling spin current polarization through non-collinear antiferromagnetism.

    abstract::The interconversion of charge and spin currents via spin-Hall effect is essential for spintronics. Energy-efficient and deterministic switching of magnetization can be achieved when spin polarizations of these spin currents are collinear with the magnetization. However, symmetry conditions generally restrict spin pola...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-17999-4

    authors: Nan T,Quintela CX,Irwin J,Gurung G,Shao DF,Gibbons J,Campbell N,Song K,Choi S-,Guo L,Johnson RD,Manuel P,Chopdekar RV,Hallsteinsen I,Tybell T,Ryan PJ,Kim J-,Choi Y,Radaelli PG,Ralph DC,Tsymbal EY,Rzchowski MS,

    更新日期:2020-09-16 00:00:00

  • Microscopic origins of the terahertz carrier relaxation and cooling dynamics in graphene.

    abstract::The ultrafast dynamics of hot carriers in graphene are key to both understanding of fundamental carrier-carrier interactions and carrier-phonon relaxation processes in two-dimensional materials, and understanding of the physics underlying novel high-speed electronic and optoelectronic devices. Many recent experiments ...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms11617

    authors: Mihnev MT,Kadi F,Divin CJ,Winzer T,Lee S,Liu CH,Zhong Z,Berger C,de Heer WA,Malic E,Knorr A,Norris TB

    更新日期:2016-05-25 00:00:00

  • Author Correction: Adaptive individual variation in phenological responses to perceived predation levels.

    abstract::An amendment to this paper has been published and can be accessed via a link at the top of the paper. ...

    journal_title:Nature communications

    pub_type: 已发布勘误

    doi:10.1038/s41467-019-13715-z

    authors: Abbey-Lee RN,Dingemanse NJ

    更新日期:2019-12-06 00:00:00