Abstract:
:In this contribution, we study situations in which nanoparticles in a fluid are strongly heated, generating high heat fluxes. This situation is relevant to experiments in which a fluid is locally heated by using selective absorption of radiation by solid particles. We first study this situation for different types of molecular interactions, using models for gold particles suspended in octane and in water. As already reported in experiments, very high heat fluxes and temperature elevations (leading eventually to particle destruction) can be observed in such situations. We show that a very simple modeling based on Lennard-Jones (LJ) interactions captures the essential features of such experiments and that the results for various liquids can be mapped onto the LJ case, provided a physically justified (corresponding state) choice of parameters is made. Physically, the possibility of sustaining very high heat fluxes is related to the strong curvature of the interface that inhibits the formation of an insulating vapor film.
journal_name
Proc Natl Acad Sci U S Aauthors
Merabia S,Shenogin S,Joly L,Keblinski P,Barrat JLdoi
10.1073/pnas.0901372106subject
Has Abstractpub_date
2009-09-08 00:00:00pages
15113-8issue
36eissn
0027-8424issn
1091-6490pii
0901372106journal_volume
106pub_type
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