Abstract:
:The development of porous carbon materials from sustainable natural sources is an attractive topic in the field of energy storage materials. This study proposed the production of nitrogen-doped porous carbon (NPC) materials from the renewable cellulose nanocrystal (CNC) as carbon source and water-soluble urea as nitrogen source without any external activation. The liquid compounding treatment and subsequent carbonization provided the NPC materials a uniform and stable N-doping (7.4% nitrogen content), high specific surface area (366.5 m2/g) and various superior electrochemical properties. The fabricated NPC sample (CU-3, with the weight ratio of 1:10 for CNC and urea) exhibited a high specific capacitance of 570.6 F/g at a current density load of 1 A/g and good cycling stability (91.2% capacitance retention after 1000 cycles at a current density of 10 A/g) in the 6 M KOH electrolyte. Applying this NPC material as the electrode component in the assembled symmetric supercapacitor demonstrated the promising electrochemical stability with the specific capacitances of 88.2 F/g at the current density of 1 A/g and capacitance retention of 99.8% after 5000 cycles. The developed N-doped porous carbon material from CNCs and urea is expected to be a sustainable electrode component for the supercapacitor materials.
journal_name
Int J Biol Macromoljournal_title
International journal of biological macromoleculesauthors
Wang S,Dong L,Li Z,Lin N,Xu H,Gao Sdoi
10.1016/j.ijbiomac.2020.09.011subject
Has Abstractpub_date
2020-12-01 00:00:00pages
4095-4103eissn
0141-8130issn
1879-0003pii
S0141-8130(20)34363-4journal_volume
164pub_type
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