Cavity-control of interlayer excitons in van der Waals heterostructures.

Abstract:

:Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterobilayer crystals promise realizations of exciton-polariton gases and condensates with inherent dipolar interactions. Here, we implement cavity-control of interlayer excitons in vertical MoSe2-WSe2 heterostructures. Our experiments demonstrate the Purcell effect for heterobilayer emission in cavity-modified photonic environments, and quantify the light-matter coupling strength of interlayer excitons. The results will facilitate further developments of dipolar exciton-polariton gases and condensates in hybrid cavity - van der Waals heterostructure systems.

journal_name

Nat Commun

journal_title

Nature communications

authors

Förg M,Colombier L,Patel RK,Lindlau J,Mohite AD,Yamaguchi H,Glazov MM,Hunger D,Högele A

doi

10.1038/s41467-019-11620-z

subject

Has Abstract

pub_date

2019-08-16 00:00:00

pages

3697

issue

1

issn

2041-1723

pii

10.1038/s41467-019-11620-z

journal_volume

10

pub_type

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