Trade-off in membrane distillation with monolithic omniphobic membranes.

Abstract:

:Omniphobic membranes are attractive for membrane distillation (MD) because of their superior wetting resistance. However, a design framework for MD membrane remains incomplete, due to the complexity of omniphobic membrane fabrication and the lack of fundamental relationship between wetting resistance and water vapor permeability. Here we present a particle-free approach that enables rapid fabrication of monolithic omniphobic membranes for MD desalination. Our monolithic omniphobic membranes display excellent wetting resistance and water purification performance in MD desalination of hypersaline feedwater containing surfactants. We identify that a trade-off exists between wetting resistance and water vapor permeability of our monolithic MD membranes. Utilizing membranes with tunable wetting resistance and permeability, we elucidate the underlying mechanism of such trade-off. We envision that our fabrication method as well as the mechanistic insight into the wetting resistance-vapor permeability trade-off will pave the way for smart design of MD membranes in diverse water purification applications.

journal_name

Nat Commun

journal_title

Nature communications

authors

Wang W,Du X,Vahabi H,Zhao S,Yin Y,Kota AK,Tong T

doi

10.1038/s41467-019-11209-6

subject

Has Abstract

pub_date

2019-07-19 00:00:00

pages

3220

issue

1

issn

2041-1723

pii

10.1038/s41467-019-11209-6

journal_volume

10

pub_type

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