Signatures of Mottness and Hundness in archetypal correlated metals.

Abstract:

:Physical properties of multi-orbital materials depend not only on the strength of the effective interactions among the valence electrons but also on their type. Strong correlations are caused by either Mott physics that captures the Coulomb repulsion among charges, or Hund physics that aligns the spins in different orbitals. We identify four energy scales marking the onset and the completion of screening in orbital and spin channels. The differences in these scales, which are manifest in the temperature dependence of the local spectrum and of the charge, spin and orbital susceptibilities, provide clear signatures distinguishing Mott and Hund physics. We illustrate these concepts with realistic studies of two archetypal strongly correlated materials, and corroborate the generality of our conclusions with a model Hamiltonian study.

journal_name

Nat Commun

journal_title

Nature communications

authors

Deng X,Stadler KM,Haule K,Weichselbaum A,von Delft J,Kotliar G

doi

10.1038/s41467-019-10257-2

subject

Has Abstract

pub_date

2019-06-20 00:00:00

pages

2721

issue

1

issn

2041-1723

pii

10.1038/s41467-019-10257-2

journal_volume

10

pub_type

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