Abstract：
:Short-wavelength luminescence is essential for high-performance optoelectronic device applications. There have been efforts to obtain intense ultraviolet (UV) emission by encapsulating ZnO one-dimensional (1D) nanostructures with materials such as ZnS. However, the encapsulation of ZnS 1D nanostructures with ZnO has not been reported. In this paper, we report ultraintense UV emission from ZnS nanorods coated with ZnO, i.e., ZnS-core/ZnO-shell nanorods. UV emission from the ZnS-core/ZnO-shell nanorods was much more intense than that obtained from the extensively studied ZnO-core/ZnS-shell nanorods. The highest intensity of the near-band-edge emission from the ZnS-core/ZnO-shell nanorods was obtained with a ZnO shell layer thickness of 35 nm, which is ∼16 times higher than that of pristine ZnS nanorods. Moreover, the deep level (DL) emission was suppressed completely. The substantial enhancement of the UV emission from the ZnS nanorods and the complete suppression of the DL emission by ZnO sheathing can be rationalized by combining the following four effects: the reinforcement of the UV emission by the overlap of the UV emissions from the ZnS core and ZnO shell, enhancement of the emission from the ZnO shell by the carrier transfer from the ZnS core to the ZnO shell, suppression of the capture of carriers by the surface states on the ZnS surface, and suppression of the visible emission and nonradiative recombination in ZnS.
journal_name
Sci Repjournal_title
Scientific reportsauthors
Lee JK,Sun GJ,Lee WS,Hyun SK,Kim KK,Choi SB,Lee Cdoi
10.1038/s41598-017-13556-0subject
Has Abstractpub_date
2017-10-12 00:00:00pages
13034issue
1issn
2045-2322pii
10.1038/s41598-017-13556-0journal_volume
7pub_type
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