Abstract:
:Transition metal oxides host a wealth of exotic phenomena ranging from charge, orbital and magnetic order to nontrivial topological phases and superconductivity. In order to translate these unique materials properties into device functionalities these materials must be doped; however, the nature of carriers and their conduction mechanism at the atomic scale remain unclear. Recent angle-resolved photoelectron spectroscopy investigations provided insight into these questions, revealing that the carriers of prototypical metal oxides undergo a transition from a polaronic liquid to a Fermi liquid regime with increasing doping. Here, by performing ab initio many-body calculations of angle-resolved photoemission spectra of titanium dioxide, we show that this transition originates from non-adiabatic polar electron-phonon coupling, and occurs when the frequency of plasma oscillations exceeds that of longitudinal-optical phonons. This finding suggests that a universal mechanism may underlie polaron formation in transition metal oxides, and provides a pathway for engineering emergent properties in quantum matter.
journal_name
Nat Communjournal_title
Nature communicationsauthors
Verdi C,Caruso F,Giustino Fdoi
10.1038/ncomms15769subject
Has Abstractpub_date
2017-06-08 00:00:00pages
15769issn
2041-1723pii
ncomms15769journal_volume
8pub_type
杂志文章abstract::Alkali metal vapors enable access to single electron systems, suitable for demonstrating fundamental light-matter interactions and promising for quantum logic operations, storage and sensing. However, progress is hampered by the need for robust and repeatable control over the atomic vapor density and over the associat...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-10158-4
更新日期:2019-05-24 00:00:00
abstract::Ensuring that one gene's transcription does not inappropriately affect the expression of its neighbors is a fundamental challenge to gene regulation in a genomic context. In plants, which lack homologs of animal insulator proteins, the mechanisms that prevent transcriptional interference are not well understood. Here ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-12328-w
更新日期:2019-09-25 00:00:00
abstract::Kevin J. Cao and Richard H. Kramer, who developed extended release with beta cyclodextrin, were inadvertently omitted from the author list and author contributions section of this Article. These errors have now been corrected in both the PDF and HTML versions of the Article. ...
journal_title:Nature communications
pub_type: 杂志文章,已发布勘误
doi:10.1038/s41467-018-03585-2
更新日期:2018-03-13 00:00:00
abstract::Energy circulation in geospace lies at the heart of space weather research. In the inner magnetosphere, the steep plasmapause boundary separates the cold dense plasmasphere, which corotates with the planet, from the hot ring current/plasma sheet outside. Theoretical studies suggested that plasmapause surface waves rel...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-15506-3
更新日期:2020-04-03 00:00:00
abstract::Hydride transfers play a crucial role in a multitude of biological redox reactions and are mediated by flavin, deazaflavin or nicotinamide adenine dinucleotide cofactors at standard redox potentials ranging from 0 to -340 mV. 2-Naphthoyl-CoA reductase, a key enzyme of oxygen-independent bacterial naphthalene degradati...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-10078-3
更新日期:2019-05-06 00:00:00
abstract::Zig-zag nanographenes are promising candidates for the applications in organic electronics due to the electronic properties induced by their periphery. However, the synthetic access to these compounds remains virtually unexplored. There is a lack in efficient and mild strategies origins in the reduced stability, incre...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-07095-z
更新日期:2018-11-12 00:00:00
abstract::Scattering-type scanning near-field optical microscopy (s-SNOM) allows spectroscopic imaging with spatial resolution below the diffraction limit. With suitable light sources, s-SNOM is instrumental in numerous discoveries at the nanoscale. So far, the light sources have been limited to continuous wave or high-repetiti...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms13212
更新日期:2016-10-17 00:00:00
abstract::The coupling of ordered electronic phases with lattice, spin, and orbital degrees of freedom are of central interest in strongly correlated systems. Their interplay has been intensively studied from femtosecond to picosecond time scales, while their dynamics beyond nanoseconds are usually assumed to follow lattice coo...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-04199-4
更新日期:2018-05-04 00:00:00
abstract::Transition metal reagents and catalysts are generally effective to cleave all three bonds (one σ and two π) in a triple bond despite its high bonding energy. Recently, chemistry of single-bond cleavage by using main-group element compounds is rapidly being developed in the absence of transition metals. However, the cl...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms5245
更新日期:2014-06-26 00:00:00
abstract::Epitaxial films may be released from growth substrates and transferred to structurally and chemically incompatible substrates, but epitaxial films of transition metal perovskite oxides have not been transferred to electroactive substrates for voltage control of their myriad functional properties. Here we demonstrate g...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-16942-x
更新日期:2020-06-24 00:00:00
abstract::Schwann cells (SCs) generate the myelin wrapping of peripheral nerve axons and are promising candidates for cell therapy. However, to date a renewable source of SCs is lacking. In this study, we show the conversion of skin fibroblasts into induced Schwann cells (iSCs) by driving the expression of two transcription fac...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms14088
更新日期:2017-02-07 00:00:00
abstract::As the desire to explore opaque materials is ordinarily frustrated by multiple scattering of waves, attention has focused on the transmission matrix of the wave field. This matrix gives the fullest account of transmission and conductance and enables the control of the transmitted flux; however, it cannot address the f...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms7893
更新日期:2015-04-20 00:00:00
abstract::Lungs resected for adenocarcinomas often harbour minute discrete foci of cytologically atypical pneumocyte proliferations designated as atypical adenomatous hyperplasia (AAH). Evidence suggests that AAH represents an initial step in the progression to adenocarcinoma in situ (AIS), minimally invasive adenocarcinoma (MI...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms9258
更新日期:2015-09-16 00:00:00
abstract::Large-scale genomic analyses of human cancers have cataloged somatic point mutations thought to initiate tumor development and sustain cancer growth. However, determining the functional significance of specific alterations remains a major bottleneck in our understanding of the genetic determinants of cancer. Here, we ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-01519-y
更新日期:2017-12-12 00:00:00
abstract::Despite progress in understanding pollination network structure, the functional roles of floral sensory stimuli (visual, olfactory) have never been addressed comprehensively in a community context, even though such traits are known to mediate plant-pollinator interactions. Here, we use a comprehensive dataset of flora...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-03448-w
更新日期:2018-03-12 00:00:00
abstract::Conventional lithium-ion batteries embrace graphite anodes which operate at potential as low as metallic lithium, subjected to poor rate capability and safety issues. Among possible alternatives, oxides based on titanium redox couple, such as spinel Li4Ti5O12, have received renewed attention. Here we further expand th...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-17233-1
更新日期:2020-07-13 00:00:00
abstract::Widely recognized as a significant carbon sink, North American forests have experienced a history of recovery and are facing an uncertain future. This growing carbon sink is dictated by recovery from land-use change, with growth trajectory modified by environmental change. To address both processes, we compiled a fore...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-05132-5
更新日期:2018-07-13 00:00:00
abstract::Gemcitabine is the first-line treatment for locally advanced and metastatic gallbladder cancer (GBC), but poor gemcitabine response is universal. Here, we utilize a genome-wide CRISPR screen to identify that loss of ELP5 reduces the gemcitabine-induced apoptosis in GBC cells in a P53-dependent manner through the Elong...
journal_title:Nature communications
pub_type: 临床试验,杂志文章
doi:10.1038/s41467-019-13420-x
更新日期:2019-12-02 00:00:00
abstract::Phospholipase C is a key enzyme in phosphoinositide turnover. Although its functions have been extensively studied at the cellular level, many questions remain concerning its functions at the organ and individual animal levels. Here we demonstrate that mice lacking phospholipase Cδ1 develop granulocytosis associated w...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms1960
更新日期:2012-07-17 00:00:00
abstract::Adolescence is a developmental period in which the mesolimbic dopaminergic "reward" circuitry of the brain, including the nucleus accumbens (NAc), undergoes significant plasticity. Dopamine D1 receptors (D1rs) in the NAc are critical for social behavior, but how these receptors are regulated during adolescence is not ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-06118-z
更新日期:2018-09-25 00:00:00
abstract::Diatoms contribute roughly 20% of global primary production, but the factors determining their ability to adapt to global warming are unknown. Here we quantify the capacity for adaptation to warming in the marine diatom Thalassiosira pseudonana. We find that evolutionary rescue under severe (32 °C) warming is slow, bu...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-03906-5
更新日期:2018-04-30 00:00:00
abstract::Epithelial-to-mesenchymal transition-like (EMT-like) is a critical process allowing initiation of metastases during tumour progression. Here, to investigate its role in intestinal cancer, we combine computational network-based and experimental approaches to create a mouse model with high metastatic potential. Construc...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms6005
更新日期:2014-10-08 00:00:00
abstract::The allotetraploid plant Nicotiana tabacum (common tobacco) is a major crop species and a model organism, for which only very fragmented genomic sequences are currently available. Here we report high-quality draft genomes for three main tobacco varieties. These genomes show both the low divergence of tobacco from its ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms4833
更新日期:2014-05-08 00:00:00
abstract::It is well known that a topologically protected gapless state appears at an interface between a topological insulator and an ordinary insulator; however, the physics of the interface between a topological insulator and a metal has largely been left unexplored. Here we report a novel phenomenon termed topological proxi...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms7547
更新日期:2015-03-12 00:00:00
abstract::Cystic fibrosis (CF) is a genetic disorder caused by defective CF Transmembrane Conductance Regulator (CFTR) function. Insulin producing pancreatic islets are located in close proximity to the pancreatic duct and there is a possibility of impaired cell-cell signaling between pancreatic ductal epithelial cells (PDECs) ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-11178-w
更新日期:2019-07-16 00:00:00
abstract::Loss of appetite or anorexia associated with inflammation impairs quality of life and increases morbidity in many diseases. However, the exact neural mechanism that mediates inflammation-associated anorexia is still poorly understood. Here we identified a population of neurons, marked by the expression of protein kina...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-10715-x
更新日期:2019-06-24 00:00:00
abstract::The original version of this Article contained an error in the spelling of the author Woochul Song, which was incorrectly given as Woochul C. Song. This has been corrected in both the PDF and HTML versions of the Article. ...
journal_title:Nature communications
pub_type: 杂志文章,已发布勘误
doi:10.1038/s41467-018-05447-3
更新日期:2018-08-14 00:00:00
abstract::The molecular mechanisms that couple glycolysis to cancer drug resistance remain unclear. Here we identify an ATP-binding motif within the NADPH oxidase isoform, NOX4, and show that ATP directly binds and negatively regulates NOX4 activity. We find that NOX4 localizes to the inner mitochondria membrane and that subcel...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-01106-1
更新日期:2017-10-19 00:00:00
abstract::The liver parenchyma is composed of hepatocytes and bile duct epithelial cells (BECs). Controversy exists regarding the cellular origin of human liver parenchymal tissue generation during embryonic development, homeostasis or repair. Here we report the existence of a hepatobiliary hybrid progenitor (HHyP) population i...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-11266-x
更新日期:2019-07-26 00:00:00
abstract::A challenge for neuroscience is to understand the conscious and unconscious processes underlying construction of willed actions. We investigated the neural substrate of human motor awareness during awake brain surgery. In a first experiment, awake patients performed a voluntary hand motor task and verbally monitored t...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-14517-4
更新日期:2020-02-04 00:00:00