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Visualization of lithium-ion transport and phase evolution within and between manganese oxide nanorods.

Abstract：

:Multiple lithium-ion transport pathways and local phase changes upon lithiation in silver hollandite are revealed via in situ microscopy including electron diffraction, imaging and spectroscopy, coupled with density functional theory and phase field calculations. We report unexpected inter-nanorod lithium-ion transport, where the reaction fronts and kinetics are maintained within the neighbouring nanorod. Notably, this is the first time-resolved visualization of lithium-ion transport within and between individual nanorods, where the impact of oxygen deficiencies is delineated. Initially, fast lithium-ion transport is observed along the long axis with small net volume change, resulting in two lithiated silver hollandite phases distinguishable by orthorhombic distortion. Subsequently, a slower reaction front is observed, with formation of polyphase lithiated silver hollandite and face-centred-cubic silver metal with substantial volume expansion. These results indicate lithium-ion transport is not confined within a single nanorod and may provide a paradigm shift for one-dimensional tunnelled materials, particularly towards achieving high-rate capability.

journal_name

Nat Commun

journal_title

Nature communications

authors

Xu F,Wu L,Meng Q,Kaltak M,Huang J,Durham JL,Fernandez-Serra M,Sun L,Marschilok AC,Takeuchi ES,Takeuchi KJ,Hybertsen MS,Zhu Y

doi

10.1038/ncomms15400

subject

Has Abstract

pub_date

2017-05-24 00:00:00

pages

15400

issn

2041-1723

pii

ncomms15400

journal_volume

8

pub_type

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