Super-resolution imaging of light-matter interactions near single semiconductor nanowires.

Abstract:

:Nanophotonics is becoming invaluable for an expanding range of applications, from controlling the spontaneous emission rate and the directionality of quantum emitters, to reducing material requirements of solar cells by an order of magnitude. These effects are highly dependent on the near field of the nanostructure, which constitutes the evanescent fields from propagating and resonant localized modes. Although the interactions between quantum emitters and nanophotonic structures are increasingly well understood theoretically, directly imaging these interactions experimentally remains challenging. Here we demonstrate a photoactivated localization microscopy-based technique to image emitter-nanostructure interactions. For a 75 nm diameter silicon nanowire, we directly observe a confluence of emission rate enhancement, directivity modification and guided mode excitation, with strong interaction at scales up to 13 times the nanowire diameter. Furthermore, through analytical modelling we distinguish the relative contribution of these effects, as well as their dependence on emitter orientation.

journal_name

Nat Commun

journal_title

Nature communications

authors

Johlin E,Solari J,Mann SA,Wang J,Shimizu TS,Garnett EC

doi

10.1038/ncomms13950

subject

Has Abstract

pub_date

2016-12-20 00:00:00

pages

13950

issn

2041-1723

pii

ncomms13950

journal_volume

7

pub_type

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