214Bi/214Pb radioactivity ratio in rainwater for residence time estimation of cloud droplets and raindrops.

Abstract:

:Continuous observation of radioactivity ratio of (214)Bi to (214)Pb as tracers in rainwater was carried out with 15-min cyclic measurement at Nagoya, Japan, from August 2011 to July 2012 to characterise wet deposition. The ratio ranged from 0.55 to 3.82. Based on the observation and a simplified time evolution model of (214)Pb and (214)Bi radioactivities during rainwater formation, the 'age' of raindrops ranged from sub-10 to several 100 min. The age would have negative correlation to rainfall intensity, but its variation for lower rainfall intensities was quite large. Secular equilibrium of (214)Pb and (214)Bi radioactivities in cloud water with airborne radon did not hold for some rainfall events.

journal_name

Radiat Prot Dosimetry

authors

Moriizumi J,Kondo D,Kojima Y,Liu H,Hirao S,Yamazawa H

doi

10.1093/rpd/ncv220

subject

Has Abstract

pub_date

2015-11-01 00:00:00

pages

55-8

issue

1-3

eissn

0144-8420

issn

1742-3406

pii

ncv220

journal_volume

167

pub_type

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