Abstract:
:Owing to the significant difference in the numbers of simulated and experimentally feasible zeolite structures, several alternative strategies have been developed for zeolite synthesis. Despite their rationality and originality, most of these techniques are based on trial-and-error, which makes it difficult to predict the structure of new materials. Assembly-Disassembly-Organization-Reassembly (ADOR) method overcoming this limitation was successfully applied to a limited number of structures with relatively stable crystalline layers (UTL, UOV, *CTH). Here, we report a straightforward, vapour-phase-transport strategy for the transformation of IWW zeolite with low-density silica layers connected by labile Ge-rich units into material with new topology. In situ XRD and XANES studies on the mechanism of IWW rearrangement reveal an unusual structural distortion-reconstruction of the framework throughout the process. Therefore, our findings provide a step forward towards engineering nanoporous materials and increasing the number of zeolites available for future applications.
journal_name
Nat Communjournal_title
Nature communicationsauthors
Kasneryk V,Shamzhy M,Zhou J,Yue Q,Mazur M,Mayoral A,Luo Z,Morris RE,Čejka J,Opanasenko Mdoi
10.1038/s41467-019-12882-3subject
Has Abstractpub_date
2019-11-12 00:00:00pages
5129issue
1issn
2041-1723pii
10.1038/s41467-019-12882-3journal_volume
10pub_type
杂志文章abstract::Radiotherapy is not currently informed by the genetic composition of an individual patient's tumour. To identify genetic features regulating survival after DNA damage, here we conduct large-scale profiling of cellular survival after exposure to radiation in a diverse collection of 533 genetically annotated human tumou...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms11428
更新日期:2016-04-25 00:00:00
abstract::CD8+ T cells provide a critical defence from pathogens at mucosal epithelia including the female reproductive tract (FRT). Mucosal immunisation is considered essential to initiate this response, however this is difficult to reconcile with evidence that antigen delivered to skin can recruit protective CD8+ T cells to m...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-09969-2
更新日期:2019-05-17 00:00:00
abstract::Oxygenic photosynthetic organisms perform solar energy conversion of water and CO2 to O2 and sugar at a broad range of wavelengths and light intensities. These cells also metabolize sugars using a respiratory system that functionally overlaps the photosynthetic apparatus. In this study, we describe the harvesting of p...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-04613-x
更新日期:2018-06-04 00:00:00
abstract::Topological defects in matter behave collectively to form highly non-trivial structures called topological textures that are characterised by conserved quantities such as the winding number. Here we show that an epitaxial ferroelectric square nanoplate of bismuth ferrite subjected to a large strain gradient (as much a...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-02813-5
更新日期:2018-01-26 00:00:00
abstract::Single-nucleotide variants that underlie phenotypic variation can affect chromatin occupancy of transcription factors (TFs). To delineate determinants of in vivo TF binding and chromatin accessibility, we introduce an approach that compares ChIP-seq and DNase-seq data sets from genetically divergent murine erythroid c...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-03082-6
更新日期:2018-02-22 00:00:00
abstract::Neural crest migration is critical to its physiological function. Mechanisms controlling mammalian neural crest migration are comparatively unknown, due to difficulties accessing this cell population in vivo. Here we report requirements of glycogen synthase kinase 3 (GSK3) in regulating the neural crest in Xenopus and...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-03512-5
更新日期:2018-03-19 00:00:00
abstract::Biomolecular X-ray structures typically provide a static, time- and ensemble-averaged view of molecular ensembles in crystals. In the absence of rigid-body motions and lattice defects, B-factors are thought to accurately reflect the structural heterogeneity of such ensembles. In order to study the effects of averaging...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms4220
更新日期:2014-01-01 00:00:00
abstract::A declining rate of recovery following disturbance has been proposed as an important early warning for impending tipping points in complex systems. Despite extensive theoretical and laboratory studies, this 'critical slowing down' remains largely untested in the complex settings of real-world ecosystems. Here, we prov...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms15811
更新日期:2017-06-09 00:00:00
abstract::Although optical technology provides the best solution for the transmission of information, all-optical devices must satisfy several qualitative criteria to be used as logic elements. In particular, cascadability is difficult to obtain in optical systems, and it is assured only if the output of one stage is in the cor...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms2734
更新日期:2013-01-01 00:00:00
abstract::Chromosomal rearrangements are essential events in the pathogenesis of both malignant and nonmalignant disorders, yet the factors affecting their formation are incompletely understood. Here we develop a zinc-finger nuclease translocation reporter and screen for factors that modulate rearrangements in human cells. We i...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms15110
更新日期:2017-04-27 00:00:00
abstract::We report color-selective photodetection from intermediate, monolayered, quantum dots buried in between amorphous-oxide semiconductors. The proposed active channel in phototransistors is a hybrid configuration of oxide-quantum dot-oxide layers, where the gate-tunable electrical property of silicon-doped, indium-zinc-o...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-00893-x
更新日期:2017-10-10 00:00:00
abstract::Carrier multiplication describes an interesting optical phenomenon in semiconductors whereby more than one electron-hole pair, or exciton, can be simultaneously generated upon absorption of a single high-energy photon. So far, it has been highly debated whether the carrier multiplication efficiency is enhanced in semi...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms2183
更新日期:2012-01-01 00:00:00
abstract::Room-temperature infrared sub-band gap photoresponse in silicon is of interest for telecommunications, imaging and solid-state energy conversion. Attempts to induce infrared response in silicon largely centred on combining the modification of its electronic structure via controlled defect formation (for example, vacan...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms4011
更新日期:2014-01-01 00:00:00
abstract::The extent to which the impact of regulatory genetic variants may depend on other factors, such as the expression levels of upstream transcription factors, remains poorly understood. Here we report a framework in which regulatory variants are first aggregated into sets, and using these as estimates of the total cis-ge...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-13762-6
更新日期:2020-01-17 00:00:00
abstract::Herpes simplex encephalitis (HSE) is the most common form of acute viral encephalitis in industrialized countries. Type I interferon (IFN) is important for control of herpes simplex virus (HSV-1) in the central nervous system (CNS). Here we show that microglia are the main source of HSV-induced type I IFN expression i...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms13348
更新日期:2016-11-10 00:00:00
abstract::14-3-3 family proteins regulate multiple signalling pathways. Understanding biological functions of 14-3-3 proteins has been limited by the functional redundancy of conserved isotypes. Here we provide evidence that 14-3-3 proteins regulate two interacting components of Tor signalling in Drosophila, translationally con...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms11501
更新日期:2016-05-06 00:00:00
abstract::RNA-binding proteins (RBPs) integrate the processing of RNAs into post-transcriptional gene regulation, but the direct contribution of them to myeloid cell specification is poorly understood. Here, we report the first global RBP transcriptomic analysis of myeloid differentiation by combining RNA-seq analysis with myel...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-01425-3
更新日期:2017-11-10 00:00:00
abstract::Crosstalk between inflammatory signalling pathways and receptor tyrosine kinases has been revealed as an indicator of cancer malignant progression. In the present study, we focus on EphA2 receptor tyrosine kinase, which is overexpressed in many human cancers. It has been reported that ligand-independent phosphorylatio...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms8679
更新日期:2015-07-09 00:00:00
abstract::Biodiversity-ecosystem functioning (BEF) experiments have shown that local species richness promotes ecosystem functioning and stability. Whether this also applies under real-world conditions is still debated. Here, we focus on larger scales of space, time and ecological organization. We develop a quasi-experimental d...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-14002-7
更新日期:2020-01-09 00:00:00
abstract::The realization that mitigation efforts to reduce carbon dioxide emissions have, until now, been relatively ineffective has led to an increasing interest in climate engineering as a possible means of preventing the potentially catastrophic consequences of climate change. While many studies have addressed the potential...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms4304
更新日期:2014-02-25 00:00:00
abstract::Perovskite light-emitting diodes (LEDs) are attracting great attention due to their efficient and narrow emission. Quasi-two-dimensional perovskites with Ruddlesden-Popper-type layered structures can enlarge exciton binding energy and confine charge carriers and are considered good candidate materials for efficient LE...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-02978-7
更新日期:2018-02-08 00:00:00
abstract::Induction of endogenous adult stem cells by administering soluble molecules provides an advantageous approach for tissue damage repair, which could be a clinically applicable and cost-effective alternative to transplantation of embryonic or pluripotent stem cell-derived tissues for the treatment of acute organ failure...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-01341-6
更新日期:2017-10-27 00:00:00
abstract::The atmosphere plays a fundamental role in the transport of microbes across the planet but it is often neglected as a microbial habitat. Although the ocean represents two thirds of the Earth's surface, there is little information on the atmospheric microbial load over the open ocean. Here we provide a global estimate ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-00110-9
更新日期:2017-08-04 00:00:00
abstract::Plants can produce organs throughout their entire life from pluripotent stem cells located at their growing tip, the shoot apical meristem (SAM). At the time of flowering, the SAM of Arabidopsis thaliana switches fate and starts producing flowers instead of leaves. Correct timing of flowering in part determines reprod...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms15120
更新日期:2017-05-17 00:00:00
abstract::The current study uses big data to study prosocial behavior by analyzing donations made on the GoFundMe platform. In a dataset of more than $44 million in online donations, we find that 21% were made while opting to be anonymous to the public, with survey results indicating that 11% of these anonymous donations (2.3% ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-11852-z
更新日期:2019-09-03 00:00:00
abstract::Predominantly, carbon atoms of various species function as acceptors of noncovalent interactions when they are part of a π-system. Here, we report on the discovery of a halogen bond involving the isocyano carbon lone pair. The co-crystallization or mechanochemical liquid-assisted grinding of model mesityl isocyanide w...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-16748-x
更新日期:2020-06-10 00:00:00
abstract::Nanostructured materials premise to revolutionize the label-free biosensing of analytes for clinical applications, leveraging the deeper interaction between materials and analytes with comparable size. However, when the characteristic dimension of the materials reduces to the nanoscale, the surface functionalization f...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-07723-8
更新日期:2018-12-10 00:00:00
abstract::Biomechanical energy harvesting textiles based on nanogenerators that convert mechanical energy into electricity have broad application prospects in next-generation wearable electronic devices. However, the difficult-to-weave structure, limited flexibility and stretchability, small device size and poor weatherability ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-08846-2
更新日期:2019-02-20 00:00:00
abstract::Solitary, persistent wave packets called solitons hold potential to transfer information and energy across a wide range of spatial and temporal scales in physical, chemical, and biological systems. Mechanical solitons characteristically emerge either as a single wave packet or uncorrelated propagating topological enti...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-13546-y
更新日期:2019-12-06 00:00:00
abstract::Plasmonics on metal-dielectric interfaces was widely seen as the main route for miniaturization of components and interconnect of photonic circuits. However recently, ultra-confined surface phonon-polaritonics in high-index chalcogenide films of nanometric thickness has emerged as an important alternative to plasmonic...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-15767-y
更新日期:2020-04-20 00:00:00