当前位置： SCI文献检索 > PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA期刊下所有文献 > Flexible, solid-state, ion-conducting membrane with 3D garnet nanofiber networks for lithium batteries.

Flexible, solid-state, ion-conducting membrane with 3D garnet nanofiber networks for lithium batteries.

Abstract：

:Beyond state-of-the-art lithium-ion battery (LIB) technology with metallic lithium anodes to replace conventional ion intercalation anode materials is highly desirable because of lithium's highest specific capacity (3,860 mA/g) and lowest negative electrochemical potential (∼3.040 V vs. the standard hydrogen electrode). In this work, we report for the first time, to our knowledge, a 3D lithium-ion-conducting ceramic network based on garnet-type Li6.4La3Zr2Al0.2O12 (LLZO) lithium-ion conductor to provide continuous Li(+) transfer channels in a polyethylene oxide (PEO)-based composite. This composite structure further provides structural reinforcement to enhance the mechanical properties of the polymer matrix. The flexible solid-state electrolyte composite membrane exhibited an ionic conductivity of 2.5 × 10(-4) S/cm at room temperature. The membrane can effectively block dendrites in a symmetric Li | electrolyte | Li cell during repeated lithium stripping/plating at room temperature, with a current density of 0.2 mA/cm(2) for around 500 h and a current density of 0.5 mA/cm(2) for over 300 h. These results provide an all solid ion-conducting membrane that can be applied to flexible LIBs and other electrochemical energy storage systems, such as lithium-sulfur batteries.

journal_name

Proc Natl Acad Sci U S A

journal_title

Proceedings of the National Academy of Sciences of the United States of America

authors

Fu KK,Gong Y,Dai J,Gong A,Han X,Yao Y,Wang C,Wang Y,Chen Y,Yan C,Li Y,Wachsman ED,Hu L

doi

10.1073/pnas.1600422113

subject

Has Abstract

pub_date

2016-06-28 00:00:00

pages

7094-9

issue

26

eissn

0027-8424

issn

1091-6490

pii

1600422113

journal_volume

113

pub_type

杂志文章

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