Abstract：
:The mechanism of droplet drying is a widely concerned fundamental issue since controlling the deposition morphology of droplet has significant influence on printing, biology pattern, self-assembling and other solution-based devices fabrication. Here we reveal a striking different kinetics-controlled deposition regime beyond the ubiquitous coffee-ring effect that suspended particles tend to kinetically accumulate at the air-liquid interface and deposit uniformly. As the interface shrinkage rate exceeds the particle average diffusion rate, particles in vertical evaporation flow will be captured by the descending surface, producing surface particle jam and forming viscous quasi-solid layer, which dramatically prevents the trapped particles from being transported to drop edge and results in uniform deposition. This simple, robust drying regime will provide a versatile strategy to control the droplet deposition morphology, and a novel direction of interface assembling for fabricating superlattices and high quality photonic crystal patterns.
journal_name
Sci Repjournal_title
Scientific reportsauthors
Li Y,Yang Q,Li M,Song Ydoi
10.1038/srep24628subject
Has Abstractpub_date
2016-04-19 00:00:00pages
24628issn
2045-2322pii
srep24628journal_volume
6pub_type
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journal_title：Scientific reports
pub_type： 已发布勘误
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更新日期：2019-12-27 00:00:00
