One Dimensional(1D)-to-2D Crossover of Spin Correlations in the 3D Magnet ZnMn2O4.

Abstract:

:We report on the intriguing evolution of the dynamical spin correlations of the frustrated spinel ZnMn2O4. Inelastic neutron scattering and magnetization studies reveal that the dynamical correlations at high temperatures are 1D. At lower temperature, these dynamical correlations become 2D. Surprisingly, the dynamical correlations condense into a quasi 2D Ising-like ordered state, making this a rare observation of two dimensional order on the spinel lattice. Remarkably, 3D ordering is not observed down to temperatures as low as 300 mK. This unprecedented dimensional crossover stems from frustrated exchange couplings due to the huge Jahn-Teller distortions around Mn(3+) ions on the spinel lattice.

journal_name

Sci Rep

journal_title

Scientific reports

authors

Disseler SM,Chen Y,Yeo S,Gasparovic G,Piccoli PM,Schultz AJ,Qiu Y,Huang Q,Cheong SW,Ratcliff W

doi

10.1038/srep17771

subject

Has Abstract

pub_date

2015-12-08 00:00:00

pages

17771

issn

2045-2322

pii

srep17771

journal_volume

5

pub_type

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