Abstract:
:Efficient and low-cost electrocatalysts for the oxygen evolution reaction are essential components of renewable energy technologies, such as solar fuel synthesis and providing a hydrogen source for powering fuel cells. Here we report that the nitrogen-doped carbon materials function as the efficient oxygen evolution electrocatalysts. In alkaline media, the material generated a current density of 10 mA cm(-2) at the overpotential of 0.38 V, values that are comparable to those of iridium and cobalt oxide catalysts and are the best among the non-metal oxygen evolution electrocatalyst. The electrochemical and physical studies indicate that the high oxygen evolution activity of the nitrogen/carbon materials is from the pyridinic-nitrogen- or/and quaternary-nitrogen-related active sites. Our findings suggest that the non-metal catalysts will be a potential alternative to the use of transition metal-based oxygen evolution catalysts.
journal_name
Nat Communjournal_title
Nature communicationsauthors
Zhao Y,Nakamura R,Kamiya K,Nakanishi S,Hashimoto Kdoi
10.1038/ncomms3390subject
Has Abstractpub_date
2013-01-01 00:00:00pages
2390issn
2041-1723pii
ncomms3390journal_volume
4pub_type
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