Abstract:
:Energy transfer of the light harvesting complex LHC-II trimer, extracted from spinach, was studied in the Q(y) region at room temperature by femtosecond transient absorption spectroscopy. Configuration interaction exciton method [Linnanto et al. (1999) J Phys Chem B 103: 8739-8750] and 2.72 A structural information reported by Liu et al. was used to calculate spectroscopic properties and excitation energy transfer rates of the complex. Site energies of the pigments and coupling constants of pigment pairs in close contact were calculated by using a quantum chemical configuration interaction method. Gaussian random variation of the diagonal and off-diagonal exciton matrix elements was used to account for inhomogeneous broadening. Rate calculations included only the excitonic states initially excited and probed in the experiments. A kinetic model was used to simulate time and wavelength dependent absorption changes after excitation on the blue side of the Q(y) transition and compared to experimentally recorded rates. Analysis of excitonic wavefunctions allowed identification of pigments initially excited and probed into later. It was shown that excitation of the blue side of the Q(y) band of a single LHC-II complex results in energy transfer from chlorophyll b's of the lumenal side to chlorophyll a's located primarly on one of the monomers of the stromal side.
journal_name
Photosynth Resjournal_title
Photosynthesis researchauthors
Linnanto J,Martiskainen J,Lehtovuori V,Ihalainen J,Kananavicius R,Barbato R,Korppi-Tommola Jdoi
10.1007/s11120-005-9004-1subject
Has Abstractpub_date
2006-03-01 00:00:00pages
267-79issue
3eissn
0166-8595issn
1573-5079journal_volume
87pub_type
杂志文章abstract::Oxygen evolving photosystem II particles were exposed to 100 and 250 W m(-2) white light at 20°C under aerobic, anaerobic and strongly reducing (presence of dithionite) conditions. Three types of photoinactivation processes with different kinetics could be distinguished: (1) The fast process which occurs under strongl...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00030061
更新日期:1990-01-01 00:00:00
abstract::Plant terpenoids are among the most diverse group of naturally-occurring organic compounds known, and several are used in contemporary consumer products. Terpene synthase enzymes catalyze complex rearrangements of carbon skeleton precursors to yield thousands of unique chemical structures that range in size from the s...
journal_title:Photosynthesis research
pub_type: 杂志文章,评审
doi:10.1007/s11120-014-9979-6
更新日期:2015-03-01 00:00:00
abstract::In thylakoid membranes, several peptides of high MW† are present which may interfere with the study of CP1's components. Modifying Cleveland's technique [7] for limited proteolysis, we have characterized the polypeptides found in the 60 kD region. Some may result from incomplete washing of the CF1 while others come fr...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00020071
更新日期:1980-03-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00033161
更新日期:1990-09-01 00:00:00
abstract::Artificial aggregates of bacteriochlorophyllc (BChlc) were formed in an aqueous medium in the presence of a lipid, monogalactosyl diglyceride (MGDG), and the optical properties of those aggregates were studied by absorption and circular dichroism (CD) mainly. Four BChlc homologs, ([E,E]BChlc F, [P,E]BChlc F, [E,M]BChl...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF02184164
更新日期:1994-07-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00029400
更新日期:1987-09-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00049278
更新日期:1985-09-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章,评审
doi:10.1007/s11120-013-9867-5
更新日期:2013-11-01 00:00:00
abstract::Analysis of leaf-level photosynthetic responses of 39 tree species grown in elevated concentrations of atmospheric CO2 indicated an average photosynthetic enhancement of 44% when measured at the growth [CO2]. When photosynthesis was measured at a common ambient [CO2], photosynthesis of plants grown at elevated [CO2] w...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00014592
更新日期:1994-03-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-014-9978-7
更新日期:2014-06-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章,评审
doi:10.1007/s11120-013-9872-8
更新日期:2014-02-01 00:00:00
abstract::Cyanobacteria, algae, and plants produce dioxygen from water. Driven and clocked by light quanta, the catalytic Mn(4)Ca Tyrosine centre accumulates four oxidizing equivalents before it abstracts four electrons from water and liberates dioxygen and protons. Intermediates of this reaction cascade are short-lived (<100 m...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-008-9321-2
更新日期:2008-10-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-012-9777-y
更新日期:2012-10-01 00:00:00
abstract::Soybean [Glycine max (L.) Merr. cv. Williams 82 and A3127] plants were grown in the field under long-term soil moisture deficit and irrigation to determine the effects of severe drought stress on the photosynthetic capacity of soybean leaves. Afternoon leaf water potentials, stomatal conductances, intercellular CO2 co...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00051735
更新日期:1990-07-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-007-9278-6
更新日期:2008-04-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-007-9246-1
更新日期:2008-02-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00032261
更新日期:1982-01-01 00:00:00
abstract::An immunological method for quantitative determination of photosynthetic fructose-1,6-bisphosphatase in crude extracts of leaves is proposed. It is based on the ELISA technique, and offers two modifications. A non-competitive technique has a higher sensitivity and is the right option for samples of low fructose-1,6-bi...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00032710
更新日期:1987-01-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00033365
更新日期:1989-08-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章,评审
doi:10.1007/s11120-018-0567-z
更新日期:2018-12-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-016-0246-x
更新日期:2016-06-01 00:00:00
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pub_type: 杂志文章
doi:10.1007/BF00035678
更新日期:1991-10-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00032356
更新日期:1981-09-01 00:00:00
abstract::A high CO2-requiring mutant of Synechocystis PCC6803 (G3) capable of Ci transport but unable to utilize the intracellular Ci pool for photosynthesis was constructed. A DNA clone of 6.1 kbp that transforms the G3 mutant to the wild-type phenotype was isolated from a Synechocystis PCC6803 genomic library. Complementatio...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00029385
更新日期:1994-02-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-010-9551-y
更新日期:2010-07-01 00:00:00
abstract::This study was conducted to more clearly define the physiological effects of PS II herbicides on chloroplast thylakoid membrane activity and composition. Barley (Hordeum vulgare L. cv Boone) was grown in hydroponic culture at 20°C in a growth chamber with a light intensity of 500 μmole photons m(-2) s(-1). Atrazine (2...
journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00028793
更新日期:1992-04-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/BF00035009
更新日期:1990-02-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1007/s11120-013-9832-3
更新日期:2013-07-01 00:00:00
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journal_title:Photosynthesis research
pub_type: 杂志文章
doi:10.1023/B:PRES.0000017179.31351.f0
更新日期:2004-01-01 00:00:00
abstract::We present here the life and work of Shmuel Malkin (1934-2017), an accomplished scientist and a gifted musician who touched the lives of many around the world. His early scientific work addressed the dynamics of light harvesting and electron transport in photosynthesis. Later, he used photoacoustic and photothermal me...
journal_title:Photosynthesis research
pub_type: 传,历史文章,杂志文章
doi:10.1007/s11120-018-0478-z
更新日期:2018-07-01 00:00:00