Abstract:
:Here, we introduce a novel concept for the fabrication of colored materials with significantly reduced dye leaching through covalent immobilization of the desired dye using plasma-generated surface radicals. This plasma dye coating (PDC) procedure immobilizes a pre-adsorbed layer of a dye functionalized with a radical sensitive group on the surface through radical addition caused by a short plasma treatment. The non-specific nature of the plasma-generated surface radicals allows for a wide variety of dyes including azobenzenes and sulfonphthaleins, functionalized with radical sensitive groups to avoid significant dye degradation, to be combined with various materials including PP, PE, PA6, cellulose, and PTFE. The wide applicability, low consumption of dye, relatively short procedure time, and the possibility of continuous PDC using an atmospheric plasma reactor make this procedure economically interesting for various applications ranging from simple coloring of a material to the fabrication of chromic sensor fabrics as demonstrated by preparing a range of halochromic materials.
journal_name
Nat Communjournal_title
Nature communicationsauthors
De Smet L,Vancoillie G,Minshall P,Lava K,Steyaert I,Schoolaert E,Van De Walle E,Dubruel P,De Clerck K,Hoogenboom Rdoi
10.1038/s41467-018-03583-4subject
Has Abstractpub_date
2018-03-16 00:00:00pages
1123issue
1issn
2041-1723pii
10.1038/s41467-018-03583-4journal_volume
9pub_type
杂志文章abstract::All common genome-wide association (GWA) methods rely on population structure correction, to avoid false genotype-to-phenotype associations. However, population structure correction is a stringent penalization, which also impedes identification of real associations. Using recent statistical advances, we developed a ne...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms13299
更新日期:2016-11-10 00:00:00
abstract::Theory, simulations and experimental results have suggested an important role of internal friction in the kinetics of protein folding. Recent experiments on spectrin domains provided the first evidence for a pronounced contribution of internal friction in proteins that fold on the millisecond timescale. However, it ha...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms2204
更新日期:2012-01-01 00:00:00
abstract::Methane cold seep systems typically exhibit extensive buildups of authigenic carbonate minerals, resulting from local increases in alkalinity driven by methane oxidation. Here, we demonstrate that modern seep authigenic carbonates exhibit anomalously low clumped isotope values (Δ47), as much as ∼0.2‰ lower than expect...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms12274
更新日期:2016-07-22 00:00:00
abstract::In the original version of this Article, financial support and contributions in manuscript preparation were not fully acknowledged. The PDF and HTML versions of the Article have now been corrected to include the following:'M.P. and P.O. would like to thank Prof. Roderick Y.H. Lim for advice during manuscript preparati...
journal_title:Nature communications
pub_type: 杂志文章,已发布勘误
doi:10.1038/s41467-018-03304-x
更新日期:2018-03-07 00:00:00
abstract::Superchiral light, generated by the interference of two counter-propagating circularly polarized light (CPL) with same frequency, opposite handedness and different intensity, exhibits enhanced dissymmetry in its interaction with chiral molecules, and has the potential for ultrasensitive detection and characterization ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-018-07533-y
更新日期:2018-11-30 00:00:00
abstract::Multiferroic bismuth ferrite, BiFeO3, offers a vast landscape to study the interplay between different ferrroic orders. Another aspect which is equally exciting, and yet underutilized, is the possibility of large-scale ordering of domains. Along with symmetry-driven bulk photovoltaic effect, BiFeO3 presents opportunit...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-20446-z
更新日期:2021-01-12 00:00:00
abstract::The ter region of the bacterial chromosome, where replication terminates, is the last to be segregated before cell division in Escherichia coli. Delayed segregation is controlled by the MatP protein, which binds to specific sites (matS) within ter, and interacts with other proteins such as ZapB. Here, we investigate t...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-17606-6
更新日期:2020-07-30 00:00:00
abstract::Oscillatory synchrony among neurons occurs in many species and brain areas, and has been proposed to help neural circuits process information. One hypothesis states that oscillatory input creates cyclic integration windows: specific times in each oscillatory cycle when postsynaptic neurons become especially responsive...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms13808
更新日期:2016-12-15 00:00:00
abstract::The sudden deterioration of patients with novel coronavirus disease 2019 (COVID-19) into critical illness is of major concern. It is imperative to identify these patients early. We show that a deep learning-based survival model can predict the risk of COVID-19 patients developing critical illness based on clinical cha...
journal_title:Nature communications
pub_type: 杂志文章,多中心研究
doi:10.1038/s41467-020-17280-8
更新日期:2020-07-15 00:00:00
abstract::Constitutive activation of Wnt/β-catenin inhibits oligodendrocyte myelination. Tcf7l2/Tcf4, a β-catenin transcriptional partner, is required for oligodendrocyte differentiation. How Tcf7l2 modifies β-catenin signalling and controls myelination remains elusive. Here we define a stage-specific Tcf7l2-regulated transcrip...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms10883
更新日期:2016-03-09 00:00:00
abstract::Tunneling is a fundamental quantum process with no classical equivalent, which can compete with Coulomb interactions to give rise to complex phenomena. Phosphorus dopants in silicon can be placed with atomic precision to address the different regimes arising from this competition. However, they exploit wavefunctions r...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-19835-1
更新日期:2020-11-30 00:00:00
abstract::In all known examples of metal-ligand (M-L) δ and φ bonds, the metal orbitals are aligned to the ligand orbitals in a "head-to-head" or "side-to-head" fashion. Here, we report two fundamentally new types of M-L δ and φ interactions; "head-to-side" δ and "side-to-side" φ back-bonding, found in complexes of metallacyclo...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-15197-w
更新日期:2020-03-25 00:00:00
abstract::Adult neural stem cells reside in a specialized niche in the subventricular zone (SVZ). Throughout life they give rise to adult-born neurons in the olfactory bulb (OB), thus contributing to neural plasticity and pattern discrimination. Here, we show that the neurovascular protein EGFL7 is secreted by endothelial cells...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms15922
更新日期:2017-06-28 00:00:00
abstract::Digital polymers with precisely ordered units acting as the coded 0- or 1-bit, are introduced as a promising option for molecular data storage. However, the pursuit of better performance in terms of high storage capacity and useful functions never stops. Herein, we propose a concept of an information-coded 2D digital ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-09957-6
更新日期:2019-04-23 00:00:00
abstract::The development of single molecule white light emitters is extremely challenging for pure phosphorescent metal-free system at room temperature. Here we report a single pure organic phosphor, namely 4-chlorobenzoyldibenzothiophene, emitting white room temperature phosphorescence with Commission Internationale de l'Écla...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-00362-5
更新日期:2017-09-04 00:00:00
abstract::Complex behaviours may be viewed as sequences of modular actions, each elicited by specific sensory cues in their characteristic timescales. From this perspective, we can construct models in which unitary behavioural modules are hierarchically placed in context of related actions. Here, we analyse antennal positioning...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-13595-3
更新日期:2019-12-06 00:00:00
abstract::Large-scale genomic analyses of human cancers have cataloged somatic point mutations thought to initiate tumor development and sustain cancer growth. However, determining the functional significance of specific alterations remains a major bottleneck in our understanding of the genetic determinants of cancer. Here, we ...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-01519-y
更新日期:2017-12-12 00:00:00
abstract::Transition metal dichalcogenides have attracted research interest over the last few decades due to their interesting structural chemistry, unusual electronic properties, rich intercalation chemistry and wide spectrum of potential applications. Despite the fact that the majority of related research focuses on semicondu...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms11038
更新日期:2016-03-14 00:00:00
abstract::Predicting ecological effects of contaminants remains challenging because of the sheer number of chemicals and their ambiguous role in biodiversity-ecosystem function relationships. We evaluate responses of experimental pond ecosystems to standardized concentrations of 12 pesticides, nested in four pesticide classes a...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-20192-2
更新日期:2020-12-10 00:00:00
abstract::Understanding the biomolecular interactions between graphene and human immune cells is a prerequisite for its utilization as a diagnostic or therapeutic tool. To characterize the complex interactions between graphene and immune cells, we propose an integrative analytical pipeline encompassing the evaluation of molecul...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-01015-3
更新日期:2017-10-24 00:00:00
abstract::In the original version of this Article, equation three contained a sign error whereby the term RT was added when it should have been subtracted. This has now been corrected in the PDF and HTML versions of the Article. ...
journal_title:Nature communications
pub_type: 杂志文章,已发布勘误
doi:10.1038/s41467-019-08556-9
更新日期:2019-02-05 00:00:00
abstract::Acoustic sensors play an important role in many areas, such as homeland security, navigation, communication, health care and industry. However, the fundamental pressure detection limit hinders the performance of current acoustic sensing technologies. Here, through analytical, numerical and experimental studies, we sho...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms6247
更新日期:2014-10-15 00:00:00
abstract::An amendment to this paper has been published and can be accessed via a link at the top of the paper. ...
journal_title:Nature communications
pub_type: 杂志文章,已发布勘误
doi:10.1038/s41467-020-17797-y
更新日期:2020-08-04 00:00:00
abstract::A fascinating but uncharacterized action of antimitotic chemotherapy is to collectively prime cancer cells to apoptotic mitochondrial outer membrane permeabilization (MOMP), while impacting only on cycling cell subsets. Here, we show that a proapoptotic secretory phenotype is induced by activation of cGAS/STING in can...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-13689-y
更新日期:2020-01-14 00:00:00
abstract::Centromeres are specified epigenetically through the deposition of the centromere-specific histone H3 variant CENP-A. However, how additional epigenetic features are involved in centromere specification is unknown. Here, we find that histone H4 Lys5 and Lys12 acetylation (H4K5ac and H4K12ac) primarily occur within the...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms13465
更新日期:2016-11-04 00:00:00
abstract::Metal halide perovskites feature crystalline-like electronic band structures and liquid-like physical properties. The crystal-liquid duality enables optoelectronic devices with unprecedented performance and a unique opportunity to chemically manipulate the structure with low energy input. In this work, we leverage the...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-19009-z
更新日期:2020-10-16 00:00:00
abstract::Protein function and dynamics are closely related; however, accurate dynamics information is difficult to obtain. Here based on a carefully assembled data set derived from experimental data for proteins in solution, we quantify backbone dynamics properties on the amino-acid level and develop DynaMine--a fast, high-qua...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/ncomms3741
更新日期:2013-01-01 00:00:00
abstract::One of the main reasons why nonlinear-optical signal processing (regeneration, logic, etc.) has not yet become a practical alternative to electronic processing is that the all-optical elements with nonlinear input-output relationship have remained inherently single-channel devices (just like their electronic counterpa...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-017-00874-0
更新日期:2017-10-12 00:00:00
abstract::As European heatwaves become more severe, summers in the United Kingdom (UK) are also getting warmer. The UK record temperature of 38.7 °C set in Cambridge in July 2019 prompts the question of whether exceeding 40 °C is now within reach. Here, we show how human influence is increasing the likelihood of exceeding 30, 3...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-020-16834-0
更新日期:2020-06-30 00:00:00
abstract::Nonbiaryl N-C atropisomer is an important structural scaffold, which is present in natural products, medicines and chiral ligands. However the direct enantioselective C-H amination to access optically pure N-C atropisomer is still difficult and rare. Here we report a π-π interaction and dual H-bond concerted control s...
journal_title:Nature communications
pub_type: 杂志文章
doi:10.1038/s41467-019-10858-x
更新日期:2019-07-11 00:00:00