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Hierarchically-structured silver nanoflowers for highly conductive metallic inks with dramatically reduced filler concentration.

Abstract：

:Silver has long been employed as an electrically conductive component, and morphology-dependent properties have been actively investigated. Here we present a novel scalable synthesis method of flower-shaped silver nanoparticles (silver nanoflowers, Ag NFs). The preferential affinity of citrate molecules on (111) surface of silver enabled spontaneous anisotropic growth of Ag NFs (bud size: 250~580 nm, single crystalline petal thickness: 9~22 nm) with high reproducibility and a high yield of >99.5%. The unique hierarchical structure resulted in coalescence of petals over 80~120 °C which was practically employed in conductive inks to construct percolation pathways among Ag NFs. The ink with only 3 wt% of Ag NFs provided two orders of magnitude greater conductivity (1.008 × 105 Scm-1), at a low curing temperature of 120 °C, compared with the silver nanoparticle ink with a much higher silver concentration (50 wt%). This extraordinary property may provide an excellent opportunity for Ag NFs for practical applications in printable and flexible electronics.

journal_name

Sci Rep

journal_title

Scientific reports

authors

C MA,K P F,Singh S,Baik S

doi

10.1038/srep34894

subject

Has Abstract

pub_date

2016-10-07 00:00:00

pages

34894

issn

2045-2322

pii

srep34894

journal_volume

6

pub_type

杂志文章

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