Abstract:
:We present a combined experimental and theoretical study of the electronic properties of close-spaced dangling-bond (DB) pairs in a hydrogen-passivated Si(001):H p-doped surface. Two types of DB pairs are considered, called "cross" and "line" structures. Our scanning tunneling spectroscopy (STS) data show that, although the spectra taken over different DBs in each pair exhibit a remarkable resemblance, they appear shifted by a constant energy that depends on the DB-pair type. This spontaneous asymmetry persists after repeated STS measurements. By comparison with density functional theory (DFT) calculations, we demonstrate that the magnitude of this shift and the relative position of the STS peaks can be explained by distinct charge states for each DB in the pair. We also explain how the charge state is modified by the presence of the scanning tunneling microscopy (STM) tip and the applied bias. Our results indicate that, using the STM tip, it is possible to control the charge state of individual DBs in complex structures, even if they are in close proximity. This observation might have important consequences for the design of electronic circuits and logic gates based on DBs in passivated silicon surfaces.
journal_name
Sci Repjournal_title
Scientific reportsauthors
Engelund M,Zuzak R,Godlewski S,Kolmer M,Frederiksen T,García-Lekue A,Sánchez-Portal D,Szymonski Mdoi
10.1038/srep14496subject
Has Abstractpub_date
2015-09-25 00:00:00pages
14496issn
2045-2322pii
srep14496journal_volume
5pub_type
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