Tuning bad metal and non-Fermi liquid behavior in a Mott material: Rare-earth nickelate thin films.

Abstract:

:Resistances that exceed the Mott-Ioffe-Regel limit (known as bad metal behavior) and non-Fermi liquid behavior are ubiquitous features of the normal state of many strongly correlated materials. We establish the conditions that lead to bad metal and non-Fermi liquid phases in NdNiO3, which exhibits a prototype bandwidth-controlled metal-insulator transition. We show that resistance saturation is determined by the magnitude of Ni eg orbital splitting, which can be tuned by strain in epitaxial films, causing the appearance of bad metal behavior under certain conditions. The results shed light on the nature of a crossover to a non-Fermi liquid metal phase and provide a predictive criterion for Anderson localization. They elucidate a seemingly complex phase behavior as a function of film strain and confinement and provide guidelines for orbital engineering and novel devices.

journal_name

Sci Adv

journal_title

Science advances

authors

Mikheev E,Hauser AJ,Himmetoglu B,Moreno NE,Janotti A,Van de Walle CG,Stemmer S

doi

10.1126/sciadv.1500797

subject

Has Abstract

pub_date

2015-11-06 00:00:00

pages

e1500797

issue

10

issn

2375-2548

pii

1500797

journal_volume

1

pub_type

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