Tunable self-healing of magnetically propelling colloidal carpets.

Abstract:

:The process of crystallization is difficult to observe for transported, out-of-equilibrium systems, as the continuous energy injection increases activity and competes with ordering. In emerging fields such as microfluidics and active matter, the formation of long-range order is often frustrated by the presence of hydrodynamics. Here we show that a population of colloidal rollers assembled by magnetic fields into large-scale propelling carpets can form perfect crystalline materials upon suitable balance between magnetism and hydrodynamics. We demonstrate a field-tunable annealing protocol based on a controlled colloidal flow above the carpet that enables complete crystallization after a few seconds of propulsion. The structural transition from a disordered to a crystalline carpet phase is captured via spatial and temporal correlation functions. Our findings unveil a novel pathway to magnetically anneal clusters of propelling particles, bridging driven systems with crystallization and freezing in material science.

journal_name

Nat Commun

journal_title

Nature communications

authors

Massana-Cid H,Meng F,Matsunaga D,Golestanian R,Tierno P

doi

10.1038/s41467-019-10255-4

subject

Has Abstract

pub_date

2019-06-04 00:00:00

pages

2444

issue

1

issn

2041-1723

pii

10.1038/s41467-019-10255-4

journal_volume

10

pub_type

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