A single microbial electrochemical system for CO2 reduction and simultaneous biogas purification, upgrading and sulfur recovery.

Abstract:

:In this work, a single microbial electrochemical system was developed for multiple goals simultaneously - CO2 reduction, biogas purification, upgrading and sulfur recovery. This system consists of a methanogen-inoculated biocathode for CO2 reduction and a ferrous ion (Fe2+)-mediated abiotic anode for hydrogen sulfide (H2S) oxidation. In the cathodic chamber, methane production rate of 20.6 ± 1.0 μmol·h-1 and high upgrading level (up to 98.3% methane content) were achieved. In the anodic chamber, H2S was completely removed and selectively converted into elemental sulfur particles. The system showed stable performance during continuous operation for treating both pure CO2 and mixed gases, with a cathodic coulombic efficiency of up to 85.2%. This simple system holds a great potential for practical application for biogas upgrading and sulfur recovery from waste water/gases.

journal_name

Bioresour Technol

journal_title

Bioresource technology

authors

Fu XZ,Li J,Pan XR,Huang L,Li CX,Cui S,Liu HQ,Tan ZL,Li WW

doi

10.1016/j.biortech.2019.122448

subject

Has Abstract

pub_date

2020-02-01 00:00:00

pages

122448

eissn

0960-8524

issn

1873-2976

pii

S0960-8524(19)31678-5

journal_volume

297

pub_type

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