Rapid screening and analysis of alpha- and gamma-emitting radionuclides in liquids using a single sample preparation procedure.

Abstract:

:A multifaceted radiochemical testing procedure has been developed to analyze a large number of liquid samples and measure a wide range of radionuclides in a short period of time. This method involves a single, unique and fast sample preparation procedure and allows sequential/concurrent determination of analytes with accuracy and precision. The same prepared sample can be selectively analyzed by gross alpha counting, gamma-ray spectroscopy, and alpha spectroscopy. This method is especially attractive in radiological emergency events where analytical data will be needed urgently as a basis for protective action. Given the simplicity and rapidity of the method, it may be suitable for field portable laboratories, which could save time and the cost associated with the transit of samples to a fixed laboratory. A 100 mL aliquot of sample was spiked with ¹³³Ba and ⁵⁹Fe tracers and subjected to a chemical separation procedure using a combined BaSO4 and Fe(OH)3 co-precipitation scheme. Then, the gross alpha-particle activity of the prepared sample was measured with a low-background gas-proportional counter, followed by the analysis of its photon-emitters using a gamma-ray spectroscopy system with high-purity intrinsic Ge detectors. Gamma-ray determination of ¹³³Ba and ⁵⁹Fe tracers was used to assess the chemical recoveries of BaSO4 and Fe(OH)3 fractions, respectively. Selectivity of the radionuclides for co-precipitation with either BaSO4 or Fe(OH)3 components was also investigated. Alpha mass-efficiency curves were derived using ²³⁰Th and ²⁴¹Am standards as alpha-calibration sources. Various mixtures of radionuclides, including ⁵⁴Mn, ⁵⁷Co, ⁶⁰Co, ⁸⁵Sr, ⁸⁸Y, ¹⁰⁹Cd, ¹¹³Sn, ¹³⁷Cs, ¹³⁹Ce, ²⁰³Hg, ²⁰⁹Po, ²²⁶Ra, ²²⁸Ra, ²³⁰Th, ²⁴¹Am, and natural uranium were used in this study. Most were quantitatively assayed with high chemical recoveries. Alpha-isotope identification and assessment of the prepared sample was achieved by alpha spectroscopy using passivated implanted planar silicon (PIPS) detectors. It has been shown that fission products could potentially be captured and analyzed by this method.

journal_name

Health Phys

journal_title

Health physics

authors

Parsa B,Henitz JB,Carter JA

doi

10.1097/HP.0b013e3181edb854

subject

Has Abstract

pub_date

2011-02-01 00:00:00

pages

152-9

issue

2

eissn

0017-9078

issn

1538-5159

pii

00004032-201102000-00004

journal_volume

100

pub_type

杂志文章
  • Radioactivity in zirconium oxide powders used in industrial applications.

    abstract::Recent work involving the decommissioning of a former ceramic manufacturing facility licensed by the Nuclear Regulatory Commission for activities involving depleted uranium oxide has uncovered the presence of unexpected high levels of natural radioactivity in non-licensed zirconium oxide powders also used in the same ...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-199106000-00009

    authors: Lischinsky J,Vigliani MA,Allard DJ

    更新日期:1991-06-01 00:00:00

  • A Case Study of the NCRP 156 Wound Model of Embedded DU Using Data From Urine Uranium Concentrations of Wounded Veterans.

    abstract::Depleted uranium (DU) munitions were initially used by the United States (U.S.) military during the first Persian Gulf War in 1991 in order to penetrate heavily armored vehicles. However, as a result of friendly fire, several U.S. military personnel received intakes from DU munitions. One of the ongoing concerns for t...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0000000000000816

    authors: Walkingstick MT,Krage ES,Brey RR

    更新日期:2018-03-01 00:00:00

  • Radon and Thoron Measured in Petrol and Gas-oil Exhaust Fumes by Using CR-39 and LR-115 II Nuclear Track Detectors: Radiation Doses to the Respiratory Tract of Mechanic Workers.

    abstract::Mechanic workers are exposed to exhaust fumes when controlling vehicle engines in motion inside repair shops. To assess radiation doses due to radon short-lived progeny from the inhalation of exhaust fumes by mechanic workers, concentrations of these radionuclides were measured in petrol (gasoline) and gas-oil exhaust...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0000000000000285

    authors: Misdaq MA,Chaouqi A,Ouguidi J,Touti R,Mortassim A

    更新日期:2015-06-01 00:00:00

  • Inhalation reference dose (RfDi): an application of interspecies dosimetry modeling for risk assessment of insoluble particles.

    abstract::Accurate extrapolation of animal toxicity data for human health risk assessment requires determination of the effective dose to the target tissue and the sensitivity of the target tissue to that dose. The methodology for deriving reference doses [the U.S. Environmental Protection Agency's (EPA) benchmark values for ga...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-198907001-00022

    authors: Jarabek AM,Menache MG,Overton JH Jr,Dourson ML,Miller FJ

    更新日期:1989-01-01 00:00:00

  • A multidetector alpha spectroscopy analysis system.

    abstract::This document describes the attributes of an alpha spectroscopy counting and analysis system called Low Level Pulse Height Analysis (LLPHA). It was developed for multi-sample alpha spectroscopy analysis. The LLPHA system is controlled by a MIK-11/2 microcomputer with 28K of memory and uses a double-density, dual flopp...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-198403000-00014

    authors: Guilmette RA,Archibeque FA

    更新日期:1984-03-01 00:00:00

  • Radiation safety considerations for the use of ²²³RaCl₂ DE in men with castration-resistant prostate cancer.

    abstract::The majority of patients with late stage castration-resistant prostate cancer (CRPC) develop bone metastases that often result in significant bone pain. Therapeutic palliation strategies can delay or prevent skeletal complications and may prolong survival. An alpha-particle based therapy, radium-223 dichloride (²²³RaC...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0b013e3182a82b37

    authors: Dauer LT,Williamson MJ,Humm J,O'Donoghue J,Ghani R,Awadallah R,Carrasquillo J,Pandit-Taskar N,Aksnes AK,Biggin C,Reinton V,Morris M,St Germain J

    更新日期:2014-04-01 00:00:00

  • Thermal Modeling for the Next Generation of Radiofrequency Exposure Limits: Commentary.

    abstract::This commentary evaluates two sets of guidelines for human exposure to radiofrequency (RF) energy, focusing on the frequency range above the "transition" frequency at 3-10 GHz where the guidelines change their basic restrictions from specific absorption rate to incident power density, through the end of the RF band at...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0000000000000671

    authors: Foster KR,Ziskin MC,Balzano Q

    更新日期:2017-07-01 00:00:00

  • 1976 Hanford americium exposure incident: psychological aspects.

    abstract::Accidents involving exposure to radiation or radioactive materials may involve an unusual degree of emotional trauma. Methods that may be employed in dealing with such trauma are discussed in relation to a specific accident in which a radiation worker was injured and seriously contaminated with 241Am. ...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-198310000-00004

    authors: Brown WR

    更新日期:1983-10-01 00:00:00

  • Assessment of the radiological impact of using fly ash in cement.

    abstract::The radiological consequences of using fly ash as a component of cement are discussed. Measurements of the activity concentrations of the fly ash and cement are reported together with measurements of emanation coefficients and exhalation rates. The radon-exhalation rate was found to be significantly lower in concrete ...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-198302000-00005

    authors: Stranden E

    更新日期:1983-02-01 00:00:00

  • Microdosimetric-based risk factors for radiation received in space activities during a trip to Mars.

    abstract::A system for evaluating quality factors, Q, based on the microdosimetric distribution of the radiation field of interest has been set up; it makes use of a specific quality function (SQF) to obtain--given microdosimetric spectra--values for Q. The advantages of a system based on lineal energy are well recognized. Furt...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-199606000-00010

    authors: Zaider M

    更新日期:1996-06-01 00:00:00

  • Dose rates for several organs in a human from contaminated soil and hot particles using the QAD computer code.

    abstract::Dose rates from contaminated soil and hot particles have been calculated for several organs of a reference human. The calculation was performed using the computer code QAD-CGGP, a point kernel code employing combinatorial geometry for the representation of the human phantom. QAD uses buildup factors based on the geome...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-199111000-00010

    authors: Tsoulfanidis N,Phillips K

    更新日期:1991-11-01 00:00:00

  • Acute Radiation-induced GI-ARS and H-ARS in a Canine Model of Mixed Neutron/Gamma Relative to Reference Co-60 Gamma Radiation: A Retrospective Study.

    abstract::Studies performed decades ago in the canine and nonhuman primate established the dose response relationships for the hematopoietic acute radiation syndrome in response to mixed neutron/gamma, x-radiation, and Co gamma radiation. There were no published studies that determined the dose response relationships for the ga...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0000000000001215

    authors: MacVittie TJ,Jackson W 3rd

    更新日期:2020-09-01 00:00:00

  • Bioassay and laboratory survey scheduling based on radioisotope inventory.

    abstract::Bioassay and laboratory survey schedules can be generated using a radioisotope inventory program. This paper discusses the use of laboratory activity, past performance and operational factors for laboratory survey frequency determination, and use of laboratory activity for bioassay scheduling. Mayo Clinic has recently...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:

    authors: Classic KL,Gross GP

    更新日期:1990-08-01 00:00:00

  • An improved model for prediction of resuspension.

    abstract::A complete, historical dataset is presented of radionuclide resuspension-factors. These data span six orders of magnitude in time (ranging from 0.1 to 73,000 d), encompass more than 300 individual values, and combine observations from events on three continents. These data were then used to derive improved, empirical ...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0b013e31821ddb07

    authors: Maxwell RM,Anspaugh LR

    更新日期:2011-12-01 00:00:00

  • Medical health physics: a review.

    abstract::Medical health physics is the profession dedicated to the protection of healthcare providers, members of the public, and patients from unwarranted radiation exposure. Medical health physicists must be knowledgeable in the principles of health physics and in the applications of radiation in medicine. Advances in medica...

    journal_title:Health physics

    pub_type: 杂志文章,评审

    doi:10.1097/00004032-200405000-00001

    authors: Vetter RJ

    更新日期:2004-05-01 00:00:00

  • External doses to humans from 137Cs in soil.

    abstract::Calculations of absorbed doses in organs of the human body and the total effective dose due to Cs in soil as a source of external exposure are presented in this work. Calculations were done using the MCNP-4B software package. The assumption was made that photons with an energy of 662 keV are emitted in a cylindrical v...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/01.HP.0000214136.56619.2d

    authors: Krstić D,Nikezić D

    更新日期:2006-09-01 00:00:00

  • Effect of Residential Radon Decay Product Dose Factor Variability on Reporting of Dose.

    abstract::Guidelines for occupational exposure to radiation are based on annual absorbed or effective dose. Guidelines for Rn exposure are currently based on air concentrations of Rn or decay products. Models of bronchial dose from decay product exposure are based on calculations that have five major parameters with parameter v...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0000000000000828

    authors: Harley NH

    更新日期:2018-04-01 00:00:00

  • Internal dose following a major nuclear war.

    abstract::The PATHWAY model results were used, in conjunction with a hypothetical major nuclear attack on the U.S., to arrive at the ratio of internal to external dose for humans from early (48 h) fallout. Considered were the four nuclides (137Cs, 89Sr, 90Sr, 131I) that account for most of the reconstructed whole-body committed...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-199201000-00004

    authors: Peterson KR,Shapiro CS

    更新日期:1992-01-01 00:00:00

  • Decay Chain Deduction of Uranium Fission Products.

    abstract::Delayed gamma spectrum is the fingerprint of uranium materials in arms control verification technology. The decay chain is simplified into basic state linear chain and excitation state linear chain to calculate and analyze the delayed gamma spectra of fission products. Formulas of the changing rule for nuclide number ...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0000000000000521

    authors: Guo H,Tian C,Wang X,Lv N,Ma M,Wei Y

    更新日期:2016-07-01 00:00:00

  • Radon calibration chamber assembly, detector accuracy, and pertinent operational findings.

    abstract::Reliable radon laboratory operations motivated the construction of three radon gas calibration chambers. One chamber is used for background calibrations while the other two cover a radon gas concentration range of 110 to >5,550 Bq m(-3) (3-150 pCi L(-1)). The chambers entered commercial service, for tertiary radon cal...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/01.HP.0000267006.55621.2f

    authors: Distenfeld CH

    更新日期:2007-08-01 00:00:00

  • Absorbed dose from traversing spherically symmetric, Gaussian radioactive clouds.

    abstract::If a large radioactive cloud is produced, sampling may require that an airplane traverse the cloud. A method to predict the absorbed dose to the aircrew from penetrating the radioactive cloud is needed. Dose rates throughout spherically symmetric Gaussian clouds of various sizes, and the absorbed doses from traversing...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-199906000-00007

    authors: Thompson JM,Poston JW Sr

    更新日期:1999-06-01 00:00:00

  • Diurnal and seasonal variations of radon levels, effects of climatic conditions, and radon exposure assessment in a former uranium metal production facility.

    abstract::Storage of radon-producing material in two silos and two waste pits is one of the major environmental and occupational issues at a former uranium production facility, now a Superfund site. In addition, up to 100 metric tons of thorium is stored on the northeast side of the site. Concentrations of radium up to 17,600 B...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-199805000-00004

    authors: Merrill EA,Akbar-Khanzadeh F

    更新日期:1998-05-01 00:00:00

  • On the discrepancy between epidemiologic studies in individuals of lung cancer and residential radon and Cohen's ecologic regression.

    abstract::There is still substantial confusion in the radiation effects community about the inherent limitations of ecologic analysis. As a result, inordinate attention has been given to the discrepant results of Cohen, in which a negative estimate is observed for the regression of county mortality rates for lung cancer on esti...

    journal_title:Health physics

    pub_type: 评论,杂志文章

    doi:10.1097/00004032-199807000-00001

    authors: Lubin JH

    更新日期:1998-07-01 00:00:00

  • The delayed pulmonary syndrome following acute high-dose irradiation: a rhesus macaque model.

    abstract::Several radiation dose- and time-dependent tissue sequelae develop following acute high-dose radiation exposure. One of the recognized delayed effects of such exposures is lung injury, characterized by respiratory failure as a result of pneumonitis that may subsequently develop into lung fibrosis. Since this pulmonary...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0b013e3182a32b3f

    authors: Garofalo M,Bennett A,Farese AM,Harper J,Ward A,Taylor-Howell C,Cui W,Gibbs A,Lasio G,Jackson W 3rd,MacVittie TJ

    更新日期:2014-01-01 00:00:00

  • Review of Cases of Occult Radiation Exposure and an Analysis of Time to Diagnosis.

    abstract::Radiation sickness is challenging to diagnose, and the diagnosis is often based on nonclinical data. In accidents where patients are not aware of their exposure to radiation (so-called "occult exposures"), a correct diagnosis can take weeks or months. The purpose of this study is to review the time to diagnosis of rad...

    journal_title:Health physics

    pub_type: 杂志文章,评审

    doi:10.1097/HP.0000000000000861

    authors: Kunkler J,Adams TG,Manger M,Casagrande R

    更新日期:2018-08-01 00:00:00

  • Parameters for modelling the interception and retention of deposits from atmosphere by grain and leafy vegetables.

    abstract::The Normalised Specific Activity (NSA), a quantity which relates the concentration of a contaminant per unit mass of vegetation to its daily rate of ground deposition, has been used as the basis for determining interception factors and retention half-lives for radioactive contaminants deposited on grain and leafy vege...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-198211000-00006

    authors: Simmonds JR,Linsley GS

    更新日期:1982-11-01 00:00:00

  • A new approach to a site radiological control manual.

    abstract::The Pantex Plant significantly revised its Radiological Control Manual to improve its usability, streamline plant procedures, and clarify conflicting guidance. This article overviews the process used to develop the new Radiological Control Manual. ...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-200202001-00007

    authors: Farrell LM

    更新日期:2002-02-01 00:00:00

  • Development of an improved dosimetry system for the workers at the Mayak Production Association.

    abstract::Databases are being created that contain verified and updated dosimetry and worker history information for workers at the Mayak Production Association. Many workers had significant external and internal exposures, particularly during the early years (1948-1952) of operation. These dosimetric and worker history data ar...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-200007000-00012

    authors: Khokhryakov V,Suslova K,Aladova E,Vasilenko E,Miller SC,Slaughter DM,Krahenbuhl MP

    更新日期:2000-07-01 00:00:00

  • Nonlinear properties of optical filters--implications for laser safety.

    abstract::Laser safety filter materials must be evaluated at various levels up to the maximum irradiances likely to be encountered, since the absorber may exhibit nonlinear properties. Extreme care is necessary around short-duration lasers due to extremely high peak irradiances in the beam. This is especially true for visible a...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/00004032-198607000-00007

    authors: Lyon TL,Marshall WJ

    更新日期:1986-07-01 00:00:00

  • Absorbed Dose Rates in Tissue from Prompt Gamma Emissions from Near-thermal Neutron Absorption.

    abstract::Prompt gamma emission data from the International Atomic Energy Agency's Prompt Gamma-ray Neutron Activation Analysis database are analyzed to determine the absorbed dose rates in tissue to be expected when natural elements are exposed in a near-thermal neutron environment. ...

    journal_title:Health physics

    pub_type: 杂志文章

    doi:10.1097/HP.0000000000000288

    authors: Schwahn SO

    更新日期:2015-10-01 00:00:00