Thermal diffusion of radon in porous media.

Abstract:

:Based on the non-intersection model of cylindrical capillaries, the mean radius of the pores of some soils and building materials are estimated. In size, the above-mentioned radii are usually of the order of the free path of gas molecules at atmospheric pressure. A review of pore size distribution data also reveals that a large fraction of concrete pores belong to Knudsen's region. This fact indicates that the thermal gradient in these media must cause gas (radon) transport. The interpretation of the experimental data concerning the rate of emanation of 222Rn from a concrete-capped source subjected to a sudden increase in temperature is given, based on irreversible thermodynamics theory. The calculations given here for radon flux, caused by concentration and thermal gradients, are in satisfactory agreement with the experimental data. It is shown that thermodiffusion can significantly contribute to radon flux in concrete. The need to include the thermodiffusion radon flux in the radon entry model is discussed.

journal_name

Radiat Prot Dosimetry

authors

Minkin L

doi

10.1093/oxfordjournals.rpd.a006360

keywords:

subject

Has Abstract

pub_date

2003-01-01 00:00:00

pages

267-72

issue

3

eissn

0144-8420

issn

1742-3406

journal_volume

106

pub_type

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