Abstract:
:In this study, a novel catalyst, S2O82--KNO3/TiO2, which has active acidic and basic sites, was prepared and used in lignin hydrocracking with a co-catalyst, Ru/C. Ru/C is an efficient hydrogenation catalyst and S2O82--KNO3/TiO2 is a dual catalyst, which could efficiently degrade lignin. This catalytic hydrogenation system can reduce solid products to less than 1%, while giving a high liquid product yield of 93%. Catalytic hydrocracking of kraft lignin at 320°C for 6h gave 93% liquid product with 0.5% solid product. Most of this liquid product was soluble in petroleum ether (60% of 93%), which is a clear liquid and comprises mainly of monomeric and dimeric degradation products. These results demonstrated that the combination of the two catalysts is an efficient catalyst for liquefaction of lignin, with little char formation (∼1%). This concept has the potential to produce valuable chemicals and fuels from lignin under moderate conditions.
journal_name
Bioresour Technoljournal_title
Bioresource technologyauthors
Wang J,Li W,Wang H,Ma Q,Li S,Chang HM,Jameel Hdoi
10.1016/j.biortech.2017.06.024subject
Has Abstractpub_date
2017-11-01 00:00:00pages
100-106eissn
0960-8524issn
1873-2976pii
S0960-8524(17)30911-2journal_volume
243pub_type
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