Abstract:
:Catalytic co-pyrolysis (CCP) of spent coffee ground (SCG) and cellulose over HZSM-5 and HY was characterized thermogravimetrically, and a catalytic pyrolysis of two samples was conducted using a tandem micro reactor that directly connected with gas chromatography-mass spectrometry. To access the more fundamental investigations on CCP, the effects of the zeolite pore structure, reaction temperature, in-situ/ex-situ reaction mode, catalyst to feedstock ratio, and the SCG and cellulose mixing ratio were experimentally evaluated. The temperature showing the highest thermal degradation rate of cellulose with SCG slightly delayed due to the interactions during the thermolysis of two samples. HZSM-5 in reference to HY produced more aromatic hydrocarbons from CCP. With respect to the reaction temperature, the formation of aromatic hydrocarbons increased with the pyrolytic temperature. Moreover, the in-situ/ex-situ reaction mode, catalyst/feedstock, and cellulose/SCG ratio were optimized to improve the aromatic hydrocarbon yield.
journal_name
Environ Resjournal_title
Environmental researchauthors
Lee HW,Farooq A,Jang SH,Kwon EE,Jae J,Lam SS,Jung SC,Park YKdoi
10.1016/j.envres.2020.109311subject
Has Abstractpub_date
2020-05-01 00:00:00pages
109311eissn
0013-9351issn
1096-0953pii
S0013-9351(20)30204-8journal_volume
184pub_type
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