Abstract:
:Impact of gas diffusion electrodes (GDEs) was evaluated in enhancing the CO2 bio-availability for its transformation to C4-organics, especially to alcohols using selective mixed culture. Observed current density was more stable (9-11 A/m2) than submerged experiments reported and significantly varied with pH and respective CO2 solubility. Uncontrolled operating pH (starting with 8.0) showed its impact on shifting/triggering alternate metabolic pathways to increase the carbon length (butyric acid) as well as producing more reduced end products, i.e. alcohols. During the experiments, CO2 was transformed initially to a mixture of volatile fatty acids dominated with formic and acetic acids, and upon their accumulation, ethanol and butanol production was triggered. Overall, 21 g/l of alcohols and 13 g/l of organic acids were accumulated in 90 days with a coulombic efficiency (CE) of 49%. Ethanol and butanol occupied respectively about 45% and 16% of total products, indicating larger potential of this technology.
journal_name
Bioresour Technoljournal_title
Bioresource technologyauthors
Srikanth S,Singh D,Vanbroekhoven K,Pant D,Kumar M,Puri SK,Ramakumar SSVdoi
10.1016/j.biortech.2018.02.058subject
Has Abstractpub_date
2018-10-01 00:00:00pages
45-51eissn
0960-8524issn
1873-2976pii
S0960-8524(18)30251-7journal_volume
265pub_type
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