Abstract:
:Four different metal-contaminated calcareous soil types, Carbonati-Perudic Cambosols (CPC), Fe-accumuli-Stagnic Anthrosols (FSA), Ochri-Aquic Cambosols (OAC) and Calci-Orthic Aridosols (COA), were investigated. The acid buffering capacity and metal-releasing behaviors of the soils were explored using an acid extraction method. Soil incubation and pot experiments were conducted to investigate changes in soil metal speciation and the enhancement of phytoextraction by soil acidification. There were several to tens of times differences in acid buffering capacities between soils. Soil calcium content may represent the major buffering system as indicated by significant linear correlations between the amount of Ca2+ released and H+ addition, and metal release into solution with H+ addition showed three stages, i.e. little release, slow release and rapid release stages. Soil carbonate-bound and Fe/Mn oxide-bound Cd and Zn decreased with the addition of H+ to all four soils, but organic matter-bound and residual metals remained unchanged. Based on the intensity of acidification, the efficiency Cd and Zn phytoextraction increased substantially with the addition of H+ in the case of the CPC but not the FSA which had a higher acid buffering capacity than the CPC. Hence, it may be concluded that the acid buffering capacity and changes in soil metal fractions with acidification of contaminated calcareous soil types should be determined before phytoextraction of these soils is attempted.
journal_name
Chemospherejournal_title
Chemosphereauthors
Wang Z,Jia M,Li Z,Liu H,Christie P,Wu Ldoi
10.1016/j.chemosphere.2020.127045subject
Has Abstractpub_date
2020-10-01 00:00:00pages
127045eissn
0045-6535issn
1879-1298pii
S0045-6535(20)31238-8journal_volume
256pub_type
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