Abstract:
:Corn was grown under greenhouse conditions in the presence of uncleaned versus cleaned municipal sewage sludge to assess the effectiveness of a chemical leaching process that uses an inorganic acid and strong oxidants to clean biosolids (i.e., to remove metals without reducing their agronomic potential). Specifically, our study analyzed physicochemical sludge from the Montreal (MSL) wastewater treatment plant (WTP) and biological sludge from the Becancour (BSL) WTP. Both biosolids were spiked with individual metals (dry weight basis): Cd (100 mg kg-1), Cu (3000 mg kg-1), and Zn (5000 mg kg-1), or their mixture. MSL biosolid enrichment led to the solubilization of added metals and removed 84-88% of Cd, 78-79% of Cu, and 79-81% of Zn. Similarly, BSL biosolid enrichment resulted in the removal of 86-88% of Cd, 80-81% of Cu, and 88-89% of Zn. The fractional distribution of metals varied between biosolids depending on their production process, stabilization, and initial metal concentration. In the MSL biosolids, only Cu partitioning was influenced by spiking, cleanup, and washing. The three metals (Cd, Cu, and Zn) occurred either in their crystalline phase or were linked to Fe oxide, organic matter, or carbonate. In the BSL biosolids, the metals that were not in their crystalline phase were only associated with Fe oxide. This study demonstrated that 99% of Cd and Cu and 97% of Zn contents remained in the soil; however, biosolid cleanup generally decreased metal concentrations in plants, leachate, and/or soil.
journal_name
Chemospherejournal_title
Chemosphereauthors
Barraoui D,Blais JF,Labrecque Mdoi
10.1016/j.chemosphere.2020.129223subject
Has Abstractpub_date
2021-03-01 00:00:00pages
129223eissn
0045-6535issn
1879-1298pii
S0045-6535(20)33420-2journal_volume
267pub_type
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