Abstract：
:Thirty-eight surface sediments and two sediment cores were collected from Yangtze River Estuary (YRE) and adjacent East China Sea (ECS) to study the distribution patterns, origins, potential transport and burden of organochlorine pesticides (OCPs) in the marginal sea. Residues of OCPs ranged from 0.190 to 5.17 ng g(-1) dry weight with a distinct "band type" pattern under the control of Yangtze River inputs and ECS circulation system. Differences in transmission media and redox conditions in situ respectively resulted in the divergent distributions of α/β-HCH and DDD/DDE. The compositional pattern analysis implied that OCPs in the inner shelf of ECS were derived from both "weathered" and fresh sources, whereas those in the outer shelf of ECS had undergone high metabolism. Concurrent with the land-sea migration, vertical profiles of sediment cores showed increasing trends or rebound since the 1990s, characteristic of two evident "jumps" of DDE+DDD/DDT and DDT/DDE ratios. Moreover, the primary distribution pattern founded for HCHs and the considerable mass inventories calculated (6.20 metric tones for OCPs) together suggested that the contaminated sediments in the studied area to be a potential source of OCPs to the global ocean.
journal_name
Chemospherejournal_title
Chemosphereauthors
Zhou S,Yang H,Zhang A,Li YF,Liu Wdoi
10.1016/j.chemosphere.2014.03.100subject
Has Abstractpub_date
2014-11-01 00:00:00pages
26-34eissn
0045-6535issn
1879-1298pii
S0045-6535(14)00460-3journal_volume
114pub_type
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