Abstract:
:Fifty five soil samples collected in the Lithuania teritory in 2011 and 2012 were analyzed for (129)I, (137)Cs and Pu isotopes in order to investigate the level and distribution of artificial radioactivity in Lithuania. The activity and atomic ratio of (238)Pu/((239,24)0)Pu, (129)I/(127)I and (131)I/(137)Cs were used to identify the origin of these radionuclides. The (238)Pu/(239+240)Pu and (240)Pu/(239)Pu ratios in the soil samples analyzed varied in the range of 0.02-0.18 and 0.18-0.24, respectively, suggesting the global fallout as the major source of Pu in Lithuania. The values of 10(-9) to 10(-6) for (129)I/(127)I atomic ratio revealed that the source of (129)I in Lithuania is global fallout in most cases though several sampling sites shows a possible impact of reprocessing releases. Estimated (129)I/(131)I ratio in soil samples from the southern part of Lithuania shows negligible input of the Chernobyl fallout. No correlation of the (137)Cs and Pu isotopes with (129)I was observed, indicating their different sources terms. Results demonstrate uneven distribution of these radionuclides in the Lithuanian territory and several sources of contamination i.e. Chernobyl accident, reprocessing releases and global fallout.
journal_name
J Environ Radioactjournal_title
Journal of environmental radioactivityauthors
Ežerinskis Ž,Hou XL,Druteikienė R,Puzas A,Šapolaitė J,Gvozdaitė R,Gudelis A,Buivydas Š,Remeikis Vdoi
10.1016/j.jenvrad.2015.09.020subject
Has Abstractpub_date
2016-01-01 00:00:00pages
166-173eissn
0265-931Xissn
1879-1700pii
S0265-931X(15)30114-4journal_volume
151 Pt 1pub_type
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