An analytically based model for the simultaneous leaching-chain decay of radionuclides from contaminated ground surface soil layers.

Abstract:

:This paper describes an analytically based method for modeling the time-dependent radionuclide areal densities of contaminated soil surface layers when the soil experiences simultaneous leaching, surface erosion and chain radioactive decay. The model is used to predict time-dependent radionuclide areal densities in a volcanic ash blanket contaminated with spent nuclear fuel particles for the purpose of assessing the risks of radiation exposure from an extrusive volcanic event near a proposed high-level waste repository at Yucca Mountain. The method uses general analytical solutions (an expansion of the Bateman equations) for calculating serial decay, including non-radioactive decay loss terms, in order to calculate time-dependent radionuclide areal densities in the ash blanket. In the presented example, 43 "key" radionuclides are tracked and their concentrations in the blanket are displayed for a 10,000-y time period following the volcanic event. Although the analysis presented herein is for modeling contaminated volcanic ash blankets, the model would work equally well for modeling time-dependent radionuclide contamination of land surfaces in, for example, site decommissioning. It is suggested that the general solutions for serial decay (with non-radioactive decay loss terms) can also be used to model the release of radionuclides from the waste packages under anticipated repository conditions.

journal_name

Health Phys

journal_title

Health physics

authors

Jarzemba MS,Manteufel RD

doi

10.1097/00004032-199712000-00006

subject

Has Abstract

pub_date

1997-12-01 00:00:00

pages

919-27

issue

6

eissn

0017-9078

issn

1538-5159

journal_volume

73

pub_type

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