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Characterization of the particulate emissions from the BP Deepwater Horizon surface oil burns.

Abstract：

:Sampling of the smoke plumes from the BP Deepwater Horizon surface oil burns led to the unintentional collection of soot particles on the sail of an instrument-bearing, tethered aerostat. This first-ever plume sampling from oil burned at an actual spill provided an opportunistic sample from which to characterize the particles' chemical properties for polycyclic aromatic hydrocarbons (PAHs), organic carbon, elemental carbon, metals, and polychlorinated dibenzodioxins/dibenzofurans (PCDDs/PCDFs) and physical properties for size and nanostructure. Thermal-optical analyses indicated that the particulate matter was 93% carbon with 82% being refractory elemental carbon. PAHs accounted for roughly 68μg/g of the PM filter mass and 5mg/kg oil burned, much lower than earlier laboratory based studies. Microscopy indicated that the soot is distinct from more common soot by its aggregate size, primary particle size, and nanostructure. PM-bound metals were largely unremarkable but PCDD/PCDF formation was observed, contrary to other's findings. Levels of lighter PCDD/PCDF and PAH compounds were reduced compared to historical samples, possibly due to volatilization or photo-oxidation.

journal_name

Mar Pollut Bull

journal_title

Marine pollution bulletin

authors

Gullett BK,Hays MD,Tabor D,Wal RV

doi

10.1016/j.marpolbul.2016.03.069

subject

Has Abstract

pub_date

2016-06-15 00:00:00

pages

216-223

issue

1

eissn

0025-326X

issn

1879-3363

pii

S0025-326X(16)30187-4

journal_volume

107

pub_type

杂志文章

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