Abstract:
:A photosensitizer tetra-α-(2,4-di-tert-butylphenoxy)-phthalocyaninato zinc [ZnPc(OAr)4] was successfully encapsulated in SiO2 nanoparticle by the microemulsion method. The photosensitized composite nanoparticle was able to degrade 2,4,6-trichlorophenol (TCP) in aqueous solution. Under visible light irradiation, the nanoparticles efficiently generated reactive oxygen species; 95.4% of TCP was degraded after 270 min of reaction. Some aromatic compounds and aliphatic carboxylic acids were detected by mass spectrometry as the reaction intermediates. The results were different from those of previously reported photocatalytic reactions, in which valence band holes or hydroxyl radicals functioned as the main oxidants. The photosensitizing composite nanoparticle is potentially applicable to the oxidation of phenol.
journal_name
Environ Technoljournal_title
Environmental technologyauthors
Jiang Z,Yang T,Zhang Y,Wang Jdoi
10.1080/09593330.2014.1002864subject
Has Abstractpub_date
2015-07-01 00:00:00pages
1643-50issue
13-16eissn
0959-3330issn
1479-487Xjournal_volume
36pub_type
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