Abstract:
:The determination of the provenance of 'unknown' plutonium material is demonstrated through a simulation study based on an isotopic fingerprinting approach. Plutonium of known provenance was considered as the 'unknown' nuclear material in order to evaluate the potential of the approach and verify its predictive capabilities. Factor analysis was used to compare the Pu isotopic composition of the 'unknown' material with Pu isotopic compositions simulating well known spent fuels from a range of commercial nuclear power stations. The provenance of the 'unknown material' is assigned to the commercial fuel with which exhibits the highest degree of similarity with respect to the Pu composition. The approach appears promising since it accurately predicted the provenance of the one 'unknown' sample considered; nevertheless, the approach is still at the development stage. Important challenging issues related to the simulation uncertainties and its testing on real laboratory samples have to be explored prior to evaluating the potential of the approach.
journal_name
J Environ Radioactjournal_title
Journal of environmental radioactivityauthors
Nicolaou Gdoi
10.1016/j.jenvrad.2008.06.001subject
Has Abstractpub_date
2008-10-01 00:00:00pages
1708-10issue
10eissn
0265-931Xissn
1879-1700pii
S0265-931X(08)00096-9journal_volume
99pub_type
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journal_title:Journal of environmental radioactivity
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journal_title:Journal of environmental radioactivity
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2010.09.002
更新日期:2011-01-01 00:00:00
abstract::The transfer of 90Sr to rice plants following its acute ground deposition was examined experimentally in a greenhouse. Lysimeters were flooded after being filled with the soil monoliths from 12 paddy fields. A solution of 90Sr was applied to the standing water in the flooded lysimeters at the pre-transplanting stage o...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2006.12.008
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2012.06.009
更新日期:2012-11-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2004.08.010
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2015.04.011
更新日期:2015-08-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章,评审
doi:10.1016/j.jenvrad.2012.03.007
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abstract::Measuring radium-226 concentration in liquid samples using radon-222 emanation remains competitive with techniques such as liquid scintillation, alpha or mass spectrometry. Indeed, we show that high-precision can be obtained without air circulation, using an optimal air to liquid volume ratio and moderate heating. Cos...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2016.03.006
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abstract::Analysis of soil redistribution and sediment sources in semiarid and arid watersheds provides information for implementing management practices to improve rangeland conditions and reduce sediment loads to streams. The purpose of this research was to develop sediment budgets and identify potential sediment sources usin...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2009.05.008
更新日期:2009-08-01 00:00:00
abstract::Transfer of radiocesium from soil to crops is an important pathway for human intake. In the period from one to two years after the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, food monitoring results showed that radiocesium concentrations in soybean (a legume) were higher than those in other annual agricult...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2017.08.016
更新日期:2018-06-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2006.02.008
更新日期:2006-01-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章,评审
doi:10.1016/j.jenvrad.2009.06.009
更新日期:2009-10-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2019.106013
更新日期:2019-11-01 00:00:00
abstract::An automated unit was developed for the in-situ extraction of radiocaesium ((137)Cs and (134)Cs) from large volumes of seawater to achieve very low detection limits. The unit was designed for monitoring of Australian ocean and coastal waters, including at ports visited by nuclear-powered warships. The unit is housed w...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2015.08.015
更新日期:2016-01-01 00:00:00
abstract::Beneficial reuse and resource recovery of produced water often require treatment to remove radium before valuable products are extracted. The radium content of the treatment waste solids and beneficial products must be accurately determined when evaluating the efficacy and social validity of such treatments. While gam...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2019.106070
更新日期:2020-01-01 00:00:00
abstract::Aerial gamma-ray surveying uses NaI(Tl) detectors mounted in small aircraft to measure gamma radiation, emitted from the earth's surface. The data are collected as gamma-ray spectra, typically with 1 s counting times, from which are derived K, U and Th concentrations in the ground. Applications of aerial surveying inc...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2004.03.028
更新日期:2004-01-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2014.04.008
更新日期:2014-09-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2012.01.025
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2018.08.004
更新日期:2018-12-01 00:00:00
abstract::Fifty five soil samples collected in the Lithuania teritory in 2011 and 2012 were analyzed for (129)I, (137)Cs and Pu isotopes in order to investigate the level and distribution of artificial radioactivity in Lithuania. The activity and atomic ratio of (238)Pu/((239,24)0)Pu, (129)I/(127)I and (131)I/(137)Cs were used ...
journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2015.09.020
更新日期:2016-01-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
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更新日期:2002-01-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2005.09.007
更新日期:2006-01-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
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更新日期:2020-10-01 00:00:00
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journal_title:Journal of environmental radioactivity
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
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更新日期:2003-01-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2018.06.003
更新日期:2018-12-01 00:00:00
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journal_title:Journal of environmental radioactivity
pub_type: 杂志文章
doi:10.1016/j.jenvrad.2009.06.024
更新日期:2009-10-01 00:00:00