Mechanism and kinetics of electrochemical degradation of uric acid using conductive-diamond anodes.

Abstract:

:Uric acid (UA) is one of the principal effluents of urine wastewaters, widely used in agriculture as fertilizer, which is potentially dangerous and biorefractory. Hence, the degradation of UA (2,6,8-trihydroxy purine) in aqueous solution of pH 3.0 has been studied by conductive-diamond electrochemical oxidation. Hydroxyl radicals formed from water oxidation at the surface of boron-doped diamond anodes were the main oxidizing agents. Effects of current density and supporting electrolyte on the degradation rate and process efficiency are assessed. Results show that the increase of current density from 20 to 60 mA cm(-2) leads to a decrease in the efficiency of the electrochemical process. In addition, the best degradation occurred in the presence of NaCl as conductive electrolyte. Interestingly, an almost total mineralization of 50 ppm UA was obtained when anodic oxidation was performed at low current densities (20 mA cm(-2)) and in the presence of NaCl. This result confirmed that the electrolysis using diamond anodes is a very interesting technology for the treatment of UA. The identification of UA transformation products was performed by high-performance liquid chromatography (HPLC). HPLC analysis of treated solutions revealed that oxalic acid and urea were the two intermediates found. Oxalic acid was the most persistent product. Based on detected intermediates and bibliographic research, a mechanism of UA mineralization by anodic oxidation has been proposed. Ionic chromatography analysis confirmed the release of [Formula: see text] and [Formula: see text] ions during UA mineralization.

journal_name

Environ Technol

journal_title

Environmental technology

authors

Dbira S,Bensalah N,Bedoui A

doi

10.1080/09593330.2016.1173115

subject

Has Abstract

pub_date

2016-12-01 00:00:00

pages

2993-3001

issue

23

eissn

0959-3330

issn

1479-487X

journal_volume

37

pub_type

杂志文章
  • Evaluation of moisture effect on low-level CO2 adsorption by ion-exchanged zeolite.

    abstract::To enhance the capture of low-level indoor CO2, a commercial zeolite (13X) was modified with alkali and alkaline earth metals using an ion-exchange method. Although the calcium-impregnated sorbent (zeo-Ca) showed the largest adsorption capacity, with a strong binding force for carbon dioxide, its regeneration by heat ...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2011.551837

    authors: Lee KM,Lim YH,Jo YM

    更新日期:2012-01-01 00:00:00

  • Effect of different concentrations of substrate in microbial fuel cells toward bioenergy recovery and simultaneous wastewater treatment.

    abstract::Microbial fuel cells (MFCS) is a promising and expanding technology able to eliminate various pollutants of wastewater while converting its chemical energy into power energy using biocatalysts. The potential application of double-chamber microbial fuel cell (DC-MFC) for chemical oxygen demand (COD) removal and generat...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2020.1772374

    authors: Rahmani AR,Navidjouy N,Rahimnejad M,Alizadeh S,Samarghandi MR,Nematollahi D

    更新日期:2020-06-11 00:00:00

  • Effective separation and sensitive determination of cyanuric acid, melamine and cyromazine in environmental water by reversed phase high-performance liquid chromatography.

    abstract::A new method for the simultaneous determination of cyanuric acid (CA), melamine (MM) and cyromazine (CM) in different water samples was developed by using reversed phase high-performance liquid chromatography diode-array detection (RP-HPLC-DAD). The conditions of HPLC were investigated and optimized. A KROMASIL C18 co...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2010.499543

    authors: Sun H,Qin X,Ge X,Wang L

    更新日期:2011-02-01 00:00:00

  • A study of two-stage anaerobic digestion of solid potato waste using reactors under mesophilic and thermophilic conditions.

    abstract::A two-stage anaerobic digestion process operated under mesophilic and thermophilic conditions was investigated for the treatment of solid potato waste to determine optimal methane yield, efficiency of operation and process stability. A solid-bed reactor was used for hydrolysis/acidification stage while an upflow anaer...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593332808618881

    authors: Parawira W,Murto M,Read JS,Mattiasson B

    更新日期:2007-11-01 00:00:00

  • Acclimation of aerobic-activated sludge degrading benzene derivatives and co-metabolic degradation activities of trichloroethylene by benzene derivative-grown aerobic sludge.

    abstract::The acclimation of aerobic-activated sludge for degradation of benzene derivatives was investigated in batch experiments. Phenol, benzoic acid, toluene, aniline and chlorobenzene were concurrently added to five different bioreactors which contained the aerobic-activated sludge. After the acclimation process ended, the...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2014.938127

    authors: Wang S,Yang Q,Bai Z,Wang S,Wang Y,Nowak KM

    更新日期:2015-01-01 00:00:00

  • Assessment of a dielectric barrier discharge plasma reactor at atmospheric pressure for the removal of bisphenol A and tributyltin.

    abstract::The ability of a laboratory-scale dielectric barrier discharge (DBD) nonthermal plasma reactor at atmospheric pressure was assessed for the removal of bisphenol A (1 mg L(-1)) and tributyltin (10 mg L(-1)) from aqueous solutions. The elimination of both the compounds followed an exponential decay equation, and a first...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2013.869624

    authors: Hijosa-Valsero M,Molina R,Bayona JM

    更新日期:2014-05-01 00:00:00

  • Study on sludge expansion during treatment of salad oil manufacturing wastewater by yeast.

    abstract::Five yeast strains, namely Rhodotorula rubra, Candida tropicalis, Candida utilis, Candida boidinii, Trichosporon cutaneum, were isolated from soil spots of a salad oil factory, and applied for continuous treatment of salad oil manufacturing wastewater. The oil and COD removal performance of the mixed cultures were com...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593332208618257

    authors: Zheng S,Yang M,Lv W,Liu F

    更新日期:2001-05-01 00:00:00

  • The effect of amount of crude oil on extent of its biodegradation in open water- and sandy beach-laboratory simulations.

    abstract::We examined the biodegradation of varying amounts of artificially weathered Alaskan North Slope crude oil in laboratory microcosm test systems that use natural seawater and simulate spills in open water and on sandy beaches. The model bioremediation treatment consisted of periodic applications of marine bacteria, sele...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330309385672

    authors: Lepo JE,Cripe CR,Kavanaugh JL,Zhang S,Norton GP

    更新日期:2003-10-01 00:00:00

  • Pretreatment of poultry manure anaerobic-digested effluents by electrolysis, centrifugation and autoclaving process for Chlorella vulgaris growth and pollutants removal.

    abstract::Different pretreatments (electrolysis, centrifugation and autoclaving) coupled with Chlorella vulgaris biological system was used for the treatment of poultry manure anaerobic-digested effluents. The pretreated effluents were used as the growth medium for algal cultivation. The pollutant removal efficiencies of the co...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2014.963695

    authors: Wang M,Wu Y,Li B,Dong R,Lu H,Zhou H,Cao W

    更新日期:2015-03-01 00:00:00

  • The biotechnological potential of the extreme halophilic archaea Haloterrigena sp. H13 in xenobiotic metabolism using a comparative genomics approach.

    abstract::Extreme halophilic archaea are thriving and dominant populations within hypersaline environments. Because of the extreme properties of the enzymes of halophilic archaea and similar metabolic abilities to their bacterial counterparts, our interests focus on their potential biotechnological applications. In this study, ...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593331003734210

    authors: Ding JY,Lai MC

    更新日期:2010-07-01 00:00:00

  • Removal efficiency of high-concentration H2S in a pilot-scale biotrickling filter.

    abstract::A pilot-scale biotrickling filter (BTF) packed with polyurethane (PU) foam was installed at one pharmaceutical factory in Zhejiang Province to study the removal of high-concentration H2S from water treatment plant. Experiments were performed at different empty bed residence times (EBRTs), H2S input load, ratio of liqu...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593332708618687

    authors: Chen JM,Jiang LY,Sha HL

    更新日期:2006-07-01 00:00:00

  • Photocatalytic degradation of p-coumaric acid over TiO2 suspensions.

    abstract::The photocatalytic degradation of p-coumaric acid, a biorecalcitrant phenolic compound typically found in olive processing and wine distillery waste waters, has been investigated in aqueous heterogeneous solutions containing semiconductor powders as photocatalysts. The disappearance of the organic molecule follows app...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593332508618424

    authors: Poulios I,Kyriacou G

    更新日期:2002-02-01 00:00:00

  • Effects of the cycle distribution on the performance of SBRs with aerobic granular biomass.

    abstract::The aerobic granular systems are mainly sequencing batch reactors where the biomass is submitted to feast-famine regimes to promote its aggregation in the form of granules. In these systems, different cycle distributions can be applied for the simultaneous removal of organic matter, nitrogen and phosphorus. In this wo...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2012.753470

    authors: Val del Río A,Morales N,Figueroa M,Mosquera-Corral A,Campos JL,Méndez R

    更新日期:2013-05-01 00:00:00

  • Optimization of a textile dye degradation in a recirculating fluidized-bed reactor using magnetite/S2O82- process.

    abstract::Optimization of Acid Orange 7 (AO7) treatment using heterogeneous Fenton-like method in a recirculating fluidized-bed reactor (FBR) was investigated by using central composite design (CCD). Natural magnetite (NM) as Fenton-like catalyst was characterized using scanning electron microscopy. A nonlinear CCD model was ob...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2016.1267804

    authors: Aghdasinia H,Arehjani P,Vahid B,Khataee A

    更新日期:2017-10-01 00:00:00

  • Impact of stress on Aeromonas diversity in tambaqui (Colossoma macropomum) and lectin level change towards a bacterial challenge.

    abstract::Tambaqui (Colossoma macropomum) is among the most cultivated fish species in tropical countries. Stress is the main cause of disease in fish farms. The genus Aeromonas is a common causative agent of fish diseases. This work reports the identification of Aeromonas species colonizing gills of C. macropomum submitted or ...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2016.1174313

    authors: Marques DS,Ferreira DA,Paiva PM,Napoleão TH,Araújo JM,Maciel Carvalho EV,Coelho LC

    更新日期:2016-12-01 00:00:00

  • Enhancing the water flux and biological treatment in bilateral influent submerged FOMBR via applying the strategy of intermittent discharging salt.

    abstract::The forward osmotic membrane bioreactor (FOMBR) is an emerging innovative technology with broad application prospects in the field of wastewater treatment. Its application is severely limited by concentration polarization, salinity accumulation, and evident water flux decline. Gradual salinity accumulation to a maximu...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2020.1730981

    authors: Lin Y,Chen Q,Wang Y,Sua K,Hao T

    更新日期:2020-02-28 00:00:00

  • High removal of chemical and biochemical oxygen demand from tequila vinasses by using physicochemical and biological methods.

    abstract::The goal of this research is to find a more effective treatment for tequila vinasses (TVs) with potential industrial application in order to comply with the Mexican environmental regulations. TVs are characterized by their high content of solids, high values of biochemical oxygen demand (BODs), chemical oxygen demand ...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2014.882960

    authors: Retes-Pruneda JL,Davila-Vazquez G,Medina-Ramírez I,Chavez-Vela NA,Lozano-Alvarez JA,Alatriste-Mondragon F,Jauregui-Rincon J

    更新日期:2014-08-01 00:00:00

  • Photoreductive degradation of CCl4 by UV-Na2SO3: influence of various factors, mechanism and application.

    abstract::Due to the strong electron-withdrawing nature of Cl atom in CCl4, CCl4 could not readily be degraded by oxidation process. In the present study, aqueous electron (eaq-), a powerful reducing agent generated in UV-Na2SO3 system, was applied to reductively degradation of CCl4. The effects of several crucial factors (e.g....

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2019.1625957

    authors: Wang Z,Liu W,Chen H,Zhang Z,Yang Z,Yang Q

    更新日期:2021-01-01 00:00:00

  • Fate and effect of xenobiotics on biodegradation processes: basis for respirometric appraisal.

    abstract::The paper mainly focused on illustrating the merit of respirometric analysis in assessing the inhibitory/toxic impact of xenobiotics on substrate biodegradation. It also evaluated biodegradation characteristics of these chemicals at continuous exposure through acclimation ofthe microbial culture. The nature and role o...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2012.655323

    authors: Orhon D,Sözen S

    更新日期:2012-07-01 00:00:00

  • Estimation of (C/N) ratio for microbial denitrification.

    abstract::Elemental balances of microbial growth have been applied to calculate (C/N) ratio in a denitrification process. The correlation between biomass yield coefficient and degree of reduction has been used to estimate the critical (C/N) ratio. It has been shown that when the degree of reduction of the substrate is lower tha...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593332708618624

    authors: Sobieszuk P,Szewczyk KW

    更新日期:2006-01-01 00:00:00

  • Isothermal drying kinetics of sewage sludge using weathered coal fly ash as adjuvant for agronomic application.

    abstract::This study aims to evaluate the effect of weathered coal fly ash (CFA) as a drying adjuvant of sewage sludge (SS) to produce a soil amendment. The high amount of SS and CFA creates a complex waste management problem in many countries, requiring more research efforts. Towards a circular economy, CFA can be viewed as an...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2019.1700311

    authors: Gomes LA,Santos AF,Lopes RJA,Góis JC,Quina MJ

    更新日期:2019-12-09 00:00:00

  • Optimization of air protection expenditures on municipal scale.

    abstract::The application of air protection methods and technologies involves considerable investment and maintenance costs. Thus, to reduce overall expenditures an economic calculation of air pollution control, should be applied. This problem is connected in special way with areas of great population of inhabitants with spatia...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330409355438

    authors: Zelinski J,Konieczynski J,Mateja-Losa E

    更新日期:2004-01-01 00:00:00

  • [Groundwater quality in an arid area of Morocco: impact of pollution on the biodiversity and relationships between crustaceans and bacteria of health interest].

    abstract::In the north of Marrakesh (Morocco), the high anthropogenic activity and the permeable nature of the geological ground makes the water of Jbilet vulnerable to contamination. The results of physico-chemical analyses conducted in 2006 showed that two groups of wells could be distinguished. Groundwater of wells located o...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330802180237

    authors: Hallam F,Yacoubi-Khebiza M,Oufdou K,Boulanouar M

    更新日期:2008-11-01 00:00:00

  • Occurrence, characterization and insecticidal activity of Bacillus thuringiensis strains isolated from argan fields in Morocco.

    abstract::Soils collected from five locations in the argan forest (an endemic plant) in Morocco were used to form the first collection of Bacillus thuringiensis (Bt) strains from this area (58 strains). Here we found that the argan forest is a major source of Bt, as 90.62% of the samples contained Bt strains. These strains prod...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2010.536789

    authors: Aboussaid H,Vidal-Quist JC,Oufdou K,El Messoussi S,Castañera P,González-Cabrera J

    更新日期:2011-08-01 00:00:00

  • Mesophilic co-digestion of palm oil mill effluent and empty fruit bunches.

    abstract::The palm oil mill industry generates palm oil mill effluent (POME) and empty fruit bunches (EFB) as by-products. This study reports the mesophilic co-digestion of POME with EFB. The biochemical methane potential (BMP) of POME and EFB was 0.397 L CH4/g volatile solids (VS) and 0.264 L CH4/g VS, respectively. In a serie...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2013.826253

    authors: Kim SH,Choi SM,Ju HJ,Jung JY

    更新日期:2013-07-01 00:00:00

  • Swelling mechanism of urea cross-linked starch-lignin films in water.

    abstract::Coating fertilizer particles with thin films is a possibility to control fertilizer release rates. It is observed that novel urea cross-linked starch-lignin composite thin films, prepared by solution casting, swell on coming into contact with water due to the increase in volume by water uptake by diffusion. The effect...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2017.1332108

    authors: Sarwono A,Man Z,Bustam MA,Subbarao D,Idris A,Muhammad N,Khan AS,Ullah Z

    更新日期:2018-06-01 00:00:00

  • Adsorption isotherm, kinetic and mechanism of expanded graphite for sulfadiazine antibiotics removal from aqueous solutions.

    abstract::The adsorption of sulfadiazine from water by expanded graphite (EG), a low cost and environmental-friendly adsorbent, was investigated. Several adsorption parameters (including the initial sulfadiazine concentration, contact time, pH of solution, ionic strength and temperature) were studied. Results of equilibrium exp...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2016.1272637

    authors: Zhang L,Wang Y,Jin S,Lu Q,Ji J

    更新日期:2017-10-01 00:00:00

  • Treatment of high-strength wastewater by Fe(2+)-activated persulphate and hydrogen peroxide.

    abstract::Ferrous ion-activated persulphate and hydrogen peroxide were studied for the treatment of real high-strength industrial effluent. The Fenton process demonstrated greater organic load removal, biodegradability improvement and toxicity reduction as well as lower treatment cost than the activated persulphate system. Howe...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2015.1069899

    authors: Kattel E,Dulova N,Viisimaa M,Tenno T,Trapido M

    更新日期:2016-01-01 00:00:00

  • Efficient removal of cytotoxic drugs from wastewater by single-stage combined photocatalysis-algae treatment process.

    abstract::In this study, the efficiency of a single-stage combined photocatalysis-algae treatment process in the removal of the anticancer drug, flutamide (FLU), from aqueous solution has been evaluated. The removal abilities of the individual blue-green alga (Anabaena sp.), nano-sized MoS2 photocatalyst under visible light irr...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2020.1725139

    authors: Kouchakpour F,Chaibakhsh N,Naeemi AS

    更新日期:2020-02-11 00:00:00

  • Batch study for Pb2+ removal by polyvinyl alcohol-biochar macroporous hydrogel bead.

    abstract::In this paper, a novel adsorbent which used polyvinyl alcohol, alginate and biochar was successfully made and been used to remove lead from aqueous solutions. Batch experiments were carried out to evaluate the adsorption capacities of Pb (II) on this bead. Experimental data were analysed by the model equations like La...

    journal_title:Environmental technology

    pub_type: 杂志文章

    doi:10.1080/09593330.2019.1642388

    authors: Wan Z,Chen D,Pei H,Liu J,Liang S,Wang X,Wu H

    更新日期:2019-07-17 00:00:00