Abstract：
:Herein, a novel paper-based chemiluminescence (CL) assay is reported using a smartphone readout for on-site and reliable analytical applications. The CL system was based on the high-performance improving effect of cobalt-imidazole metal-organic framework (CoMOF) on luminol-hydrogen peroxide (H2O2) CL emission. The CoMOF was grown on paper and used as a support for the CL reaction, which led to an intense CL emission and good reproducibility. More importantly, the stability of luminol, as the CL reagent, was greatly improved in the presence of CoMOF. This high stability, along with the high-yield CL emission, makes the device highly suitable for commercialization. Furthermore, using a smartphone as the detector for the developed device made the process easier and more accessible for public usage. In this work, the new paper-based CL smartphone device was used for the detection of the total phenolic content of food samples. Phenolic compounds (PC) are hydroxyl radical scavengers that can effectively quench the CL emission of the luminol-H2O2-CoMOF system. After optimizing the reaction conditions, the system could detect PC at the μg mL-1 level. Detection limits of 0.12, 0.28, 0.46, 0.85, and 1.23 μg mL-1 were obtained for gallic acid, quercetin, catechin, kaempferol, and caffeic acid, respectively. This work is the first report on the practical application of smartphone CL assays for the estimation of PC. The proposed assay is an easy-to-use, low-cost, portable, and suitable assay for on-site screening purposes.
journal_name
Talantajournal_title
Talantaauthors
Al Lawati HAJ,Hassanzadeh J,Bagheri N,Al Lawati Idoi
10.1016/j.talanta.2021.122648keywords:
["Antioxidants","Chemiluminescence","Food products","Metal-organic framework","Sensor","Smartphone detector"]subject
Has Abstractpub_date
2021-11-01 00:00:00pages
122648eissn
0039-9140issn
1873-3573pii
S0039-9140(21)00569-5journal_volume
234pub_type
杂志文章相关文献
文献大全abstract：:Carbohydrates are an indispensable part of early life evolution. The determination of their structures is a key step to analyze their critical roles in biological systems. A variation of composition, glycosidic linkage, and (or) configuration between carbohydrate isomers induces structure diversity and brings challeng...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122348
更新日期：2021-08-01 00:00:00
abstract：:Column technology is an important part in capillary electrochromatographic science. Developing novel stationary phase with high separation efficiency and high loading capacity is an essential work. In this work, a novel spherical vinyl-functionalized covalent-organic framework (COF-V) was synthesized at room temperatu...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122330
更新日期：2021-08-01 00:00:00
abstract：:In this paper, a novel vortex assisted solid phase extraction procedure combined with inductively coupled plasma optic emission spectrometry was presented for determination of Mn, Cu, Ni, Cr, Cd and Pb directly in oily matrix. The suggested separation and preconcentration method was based on simultaneous sorption of t...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122312
更新日期：2021-08-01 00:00:00
abstract：:With a growing interest in precise and sensitive diagnosis for criminal investigations, nanoparticles (NPs) have intrigued scientific minds working in the field of forensic science due to their exceptional properties. Magnetic nanoparticles (MNPs) have emerged as a powerful tool for improving forensic analysis due to ...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122297
更新日期：2021-08-01 00:00:00
abstract：:There is a growing need for real-time monitoring of metabolic products that could reflect cell damages over extended periods. In this paper, we report the design and development of an original multiparametric (bio)sensing platform that is tailored for the real-time monitoring of cell metabolites derived from cell cult...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122275
更新日期：2021-07-01 00:00:00
abstract：:It is widely accepted that cancer, the second leading cause of death, is a morbidity with big impacts on the global health. In the last few years, chemo-therapeutic treatment continually induces alone most lengthy consequents, which is extremely harmful for the physiological and psychological health of the patients. I...
journal_title：Talanta
pub_type： 杂志文章,评审
doi：10.1016/j.talanta.2021.122247
更新日期：2021-07-01 00:00:00
abstract：:Industrial hemp (Cannabis sativa L.) represents an important plant, used for a variety of uses including pharmaceutical and nutraceutical purposes. As such, a detailed characterization of the composition of this plant could help future research to further exploit the beneficial effects of hemp compounds on the human h...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122249
更新日期：2021-06-01 00:00:00
abstract：:A sensitive and highly reproducible cardiac troponin I (cTnI) immunoassay in human serum is a challenging research goal for researchers studying biosensors because cTnI can undergo proteolysis and various modifications in blood. Furthermore, the reproducible detection of cTnI at very low concentrations is also require...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122233
更新日期：2021-06-01 00:00:00
abstract：:In this research, a novel Ag3PO4 NPs@MoS2 nanosheet-based electrochemiluminescence (ECL) sensing system was developed to provide an effective method for tumor gene detection. At first, fluorine, sulfur-doped BN quantum dot (F, S-BN QD) were prepared as ECL emitter. Sulfur dopant can provide more reactive sites in the ...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122221
更新日期：2021-06-01 00:00:00
abstract：:The thiolysis of 7-nitro-1,2,3-benzoxadiazole amine (NBD-A) paves the way for specific sensing of H2S over biothiols and real-time imaging in living organisms. Rational fabrication of NBD-A-based probe with ratiometric mode and two-photon excitation is highly appealing to achieve high quality bioimaging. In this work,...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122269
更新日期：2021-06-01 00:00:00
abstract：:A hapten-protein conjugate with copper nanoparticles (Hap-Car-BSA@CuNPs) was first synthesized in the present work for the determination of carbaryl. The copper nanoparticles (CuNPs) of the conjugate were used as electrochemical labels in the direct solid-phase competitive determination of carbaryl residues in flour f...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122174
更新日期：2021-06-01 00:00:00
abstract：:The aim of this work was to select and identify the best markers of aromatic hydrocarbon mineral oil (MOAH) in food packaging. For this purpose, a series of mineral oils was initially analysed. Polycyclic Aromatic Hydrocarbons (PAHs) and the alkylated isomers of Methylnaphthalene (MNS), Diisopropylnaphtalene (DIPNs), ...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.122079
更新日期：2021-05-15 00:00:00
abstract：:Cellular differentiation is a fundamental process in which one cell type changes into one or more specialized cell types. Cellular differentiation starts at the beginning of embryonic development when a simple zygote begins to transform into a complex multicellular organism composed of various cell and tissue types. T...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122164
更新日期：2021-05-15 00:00:00
abstract：:Significant improvements in the voltammetric determination of β-carotene (BCA) have been achieved, mainly by the replacement of toxic dichloromethane with acetone and using non-mercury electrode. The respective procedure is based on anodic oxidation of BCA at a gold electrode in the disc configuration, when using squa...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122088
更新日期：2021-05-15 00:00:00
abstract：:Exosomes (30-200 nm) play important roles in intercellular communication. Because their contents differ between healthy individuals and subjects diagnosed with various diseases, exosomes have been regarded as potential sources of biomarkers for clinical diagnosis. However, the accuracy of diagnosis by exosomal biomark...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122186
更新日期：2021-05-01 00:00:00
abstract：:Ferrites have attracted considerable attention in biosensor developments owing to their favorable electrochemical and magnetic properties. Speedy and trace analysis can be succeeded by the sensors based on magnetic nanohybrids. In this work, we reported a novel method for one-step synthesis of magnetic ferrites compos...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122165
更新日期：2021-05-01 00:00:00
abstract：:Nucleic acid detection is of great importance in a variety of areas, from life science and clinical diagnosis to environmental monitoring and food safety. Unfortunately, nucleic acid targets are always found in trace amounts and their response signals are difficult to be detected. Amplification mechanisms are then pra...
journal_title：Talanta
pub_type： 杂志文章,评审
doi：10.1016/j.talanta.2021.122146
更新日期：2021-05-01 00:00:00
abstract：:A novel sandwich-type electrochemical immunosensor has been fabricated for simultaneous determination of three kinds of tumor markers (TMs). The signal-amplified platform for sensor was assisted by graphene oxide (GO) loaded with Poly(styrene-alt-maleic anhydride) (PSMA). Three TMs of prostate specific antigen (PSA), ...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122133
更新日期：2021-05-01 00:00:00
abstract：:An electronic nose, comprising nine metal oxide sensors, has been built aiming to classify olive oils according to the fruity intensity commercial grade (ripely fruity or light, medium and intense greenly fruity), following the European regulated complementary terminology. The lab-made sensor device was capable to dif...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122122
更新日期：2021-05-01 00:00:00
abstract：:In the present work, the exceptional electrochemical properties of carbon paper were characterized and explored in the development of a sensor for the anti-inflammatory drug, ketoprofen. An initial electrochemical characterization of the carbon paper with a redox indicator revealed much higher voltammetric peaks in co...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122111
更新日期：2021-05-01 00:00:00
abstract：:Temperature changes in cells are generally accompanied by physiological processes. Cellular temperature measurements can provide important information to fully understand cellular mechanisms. However, temperature measurements with conventional methods, such as fluorescent polymeric thermometers and thermocouples, have...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122101
更新日期：2021-05-01 00:00:00
abstract：:The reliable determination of the Ag(I) affinity for biomolecules is an essential issue in the fields of structural analysis and sensor design. However, the urgent problem confronting researchers is lack of a direct and accurate Ag(I) affinity evaluation as a reference standard for ligand analysis. We communicated her...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122089
更新日期：2021-05-01 00:00:00
abstract：:A tandem ion mobility spectrometer was used to mobility isolate ions at the drift time for trinitrotoluene (TNT) in a first mobility stage, remove an interfering compound by ion decomposition in a middle reactive stage, and mobility characterize the remaining TNT ions in a second mobility stage. This sequential proces...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.121944
更新日期：2021-05-01 00:00:00
abstract：:Semiconductor quantum dots (QDs) are one of the most popular luminescent labels that are widely used in food and medical analysis. Their unique optical properties establish QDs as excellent tools for highly sensitive biosensors based on Förster resonance energy transfer (FRET). To provide a convenient analytical syste...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.121973
更新日期：2021-04-01 00:00:00
abstract：:A novel magnetic C3N5 framework material (Fe3O4/C3N5) was developed as a high selectivity extractant for La(III) determination in food samples. The Fe3O4/C3N5 material was synthesized by thermal deammoniation method and has larger surface area (100.3 m2 g-1) and more effective adsorption sites compared with that of in...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2021.122086
更新日期：2021-04-01 00:00:00
abstract：:Increasing accounts of fraud and persistent labeling problems have brought the authenticity of leather products into question. In this study, we developed an extremely simplified workflow for real-time, in situ, and unambiguous authentication of leather samples using rapid evaporative ionization mass spectrometry (REI...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.122069
更新日期：2021-04-01 00:00:00
abstract：:The determination of low abundant endogenous components is a challenge for the clinical samples. Histamine, a crucial endogenous component, fulfils various regulatory and mediatory functions in human, and the change of content is a critical index for the diagnosis of some diseases, especially allergy, asthma, and anap...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.122056
更新日期：2021-04-01 00:00:00
abstract：:A tutorial and spreadsheet for the validation and bottom-up uncertainty evaluation of quantifications performed by instrumental methods of analysis based on linear weighted calibrations is presented. The developed tool automatically assesses if calibrator values uncertainty is negligible given instrumental signal prec...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.122044
更新日期：2021-04-01 00:00:00
abstract：:Silver-based nanoparticles (Ag-b-NPs) are currently a cause for concern because they are being produced in increasing quantities for use in industrial goods and consumer products. This goes hand in hand with their release to the environment and the resultant risks for the entire ecosystem. Therefore, it is essential t...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.122028
更新日期：2021-04-01 00:00:00
abstract：:A chemical imaging method to mass surveil bacteria cells among plant tissues in situ is reported. Bacteria cells were pre-labeled with 3-mercaptophenylboronic acid for complexation with gold nanoparticles. Surface-enhanced Raman spectra were collated en masse to generate panoramic chemical images of bacteria populatio...
journal_title：Talanta
pub_type： 杂志文章
doi：10.1016/j.talanta.2020.122008
更新日期：2021-04-01 00:00:00
