Abstract:
:Polycyclic aromatic hydrocarbons (PAHs) are with great environmental concerns due to their toxic, mutagenic, and carcinogenic properties. The harmful effects caused by PAHs emitted from indoor sources may be more direct and serious. In this study, PAHs in aerosol from two typical indoor sources, the cooking fume (CF) and environmental tobacco smoke (ETS) were collected by simulation emission in a chamber. Eighteen PAHs were analyzed by GC/MS and GC/C/IRMS. The chemical profiles of these two sources were described. Results indicated that Fluoranthene, Pyrene and Fluorene in CF, and Fluorene, Phenanthrene, Indeno(1,2,3-cd)pyrene and Benz(a)anthracene in ETS, relative quantity of which were variable in a smaller range, can be regarded as tracers of indoor PAHs sources. There are distinct differences among the ratios of Benz(a)anthracene/Chrysene, Benzo(e)pyrene/Benzo(a)pyrene and Indeno(1,2,3-cd)pyrene/Benzo(g,h,i)perylene between CF and EST. Distribution of delta(13)C of individual PAHs in ETS samples ranged from -21.76 per thousand to -29.32 per thousand, wider than that in CF samples (-22.94 per thousand to -28.39 per thousand). The delta(13)C of Phenanthrene, Benz(a)anthracene, Benzo(b)fluoranthene, Benzo(k)fluoranthene and Indeno(1,2,3-cd)pyrene between these two sources showed great differences. The (13)C was enriched in low molecule weight compounds of CF samples and in high molecule weight compounds of ETS samples.
journal_name
Chemospherejournal_title
Chemosphereauthors
Zhang L,Bai Z,You Y,Wu J,Feng Y,Zhu Tdoi
10.1016/j.chemosphere.2008.12.063subject
Has Abstractpub_date
2009-04-01 00:00:00pages
453-61issue
4eissn
0045-6535issn
1879-1298pii
S0045-6535(08)01592-0journal_volume
75pub_type
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