Abstract:
:Fly ash and Air Pollution Control (APC) residues collected from three municipal solid waste incinerators in Denmark and Greenland were treated by electrodialytic remediation at pilot scale for 8-10 h. This work presents for the first time the effect of electrodialytic treatment on polychlorinated dibenzo-p-dioxins (PCDD) and polychlorinated dibenzofurans (PCDF), and how these levels impact on the valorization options for fly ash and APC residue. PCDD/PCDF levels in the original residues ranged between 4.85 and 197 ng g(-1), being higher for the electrostatic precipitator fly ash. The toxic equivalent (TEQ) varied ten fold, ranging 0.18-2.0 ng g(-1) I-TEQ, with penta and hexa-homologs being most significant for toxicity. After the electrodialytic treatment PCDD/PCDF levels increased in the residues (between 1.4 and 2.0 times). This does not mean PCDD/PCDF were synthesized, but else that soluble materials dissolve, leaving behind the non-water soluble compounds, such as PCDD/PCDF. According to the Basel Convention, PCDD/PCDF levels in these materials is low (<15 μg WHO-TEQ kg(-1)) and the fly ash and APC residue could eventually be valorized, for instance as construction material, provided end-of-waste criteria are set and that a risk assessment of individual options is carried out, including the end-of-life stage when the materials become waste again.
journal_name
Chemospherejournal_title
Chemosphereauthors
Dias-Ferreira C,Kirkelund GM,Jensen PEdoi
10.1016/j.chemosphere.2016.01.061subject
Has Abstractpub_date
2016-04-01 00:00:00pages
380-7eissn
0045-6535issn
1879-1298pii
S0045-6535(16)30060-1journal_volume
148pub_type
杂志文章相关文献
CHEMOSPHERE文献大全abstract::A simple and relatively fast approach for developing a solid phase extraction has been described and used for determination of trace quantities of some heavy and transition metal ions with sodium dodecyl sulfate (SDS)-coated poly vinyl chloride (PVC) modified with bis(2-hydroxyacetophenone)-1,4-butanediimine (BHABDI) ...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2008.09.034
更新日期:2009-01-01 00:00:00
abstract::Tembotrione is a rather novel pesticide, usually used for post-emergence weed control. Even though its use is rapidly growing, it is not followed by an adequate flow of scientific evidence regarding its toxicity towards non-target organisms. We evaluated the potential of low doses of tembotrione to induce oxidative st...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2020.126643
更新日期:2020-08-01 00:00:00
abstract::This study evaluated the effect of humic acid (HA) on physicochemical properties of bacterial surfaces and on mass transfer of polycyclic aromatic hydrocarbons (PAHs) from aqueous phase into intracellular bacteria. Due to this process' potential for bacterial degradation, using Sphingobium sp. PHE3, degradation of phe...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2017.06.026
更新日期:2017-10-01 00:00:00
abstract::With the main objective of improving the removal of nitrogen from domestic wastewater and more sustainably, a moving bed and constructed wetland (MBCW) integrated bioreactor was fabricated and evaluated with continuous and intermittent aeration operations. The hybrid system achieves average removal efficiencies up to ...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2020.127744
更新日期:2020-12-01 00:00:00
abstract::Chronic ototoxicity of β-diketone antibiotics (DKAs) to zebrafish (Danio rerio) was explored in detail by following abnormal expressions of two hearing-related miRNAs. Dose-dependent down-regulation of miR-96 and miR-184 was observed in otoliths during embryonic-larval development. Continuous DKA exposure to 120-hpf l...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2018.09.118
更新日期:2019-01-01 00:00:00
abstract::There is growing concern regarding human dietary exposure to arsenic (As) via consumption of rice. The concentration and speciation of As in rice are highly variable, and models describing rice As speciation as a function of environmental covariates remain elusive. We conducted a survey of paddy rice and soil in the M...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2020.129092
更新日期:2021-02-01 00:00:00
abstract::Natural zeolite and synthetic zeolite, MCM-22, were employed as effective adsorbents for a basic dye, methylene blue, removal from wastewater. Two methods, Fenton oxidation and high temperature combustion, have been used for regeneration of used materials. It is found that MCM-22 exhibits equilibrium adsorption at 1.7...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2006.02.043
更新日期:2006-09-01 00:00:00
abstract::Release of 3,3'-dichlorobenzidine (DCB), an intermediate in dye manufacturing processes, is of environmental concern due to its carcinogenic nature. An 11-year field study has been conducted to elucidate the fate and behavior of DCB and its congeners in the Lake Macatawa (Holland, MI, USA) sediment-water system. The s...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2004.09.081
更新日期:2005-02-01 00:00:00
abstract::Bioaccumulation models take various elimination and uptake processes into account, estimating rates from chemical lipophilicity, expressed as the octanol-water partition ratio (K(ow)). Here, we focussed on metabolism, which transforms parent compounds into usually more polar metabolites, thus enhancing elimination. Th...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2012.03.033
更新日期:2012-08-01 00:00:00
abstract::In order to assess the influence of the aromatic substitution on the ability of a soil bacterial strain, Arthrobacter sp. N2, to degrade phenylurea herbicides, biotransformation assays were performed in mineral medium with resting cells of this soil bacterial strain on three phenylurea herbicides (diuron, chlorotoluro...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/s0045-6535(01)00193-x
更新日期:2002-01-01 00:00:00
abstract::The intricacy in the treatment of effluents from the textile sector attracts the researchers since 20th century. Dye intermediate manufacturing industries are responsible for producing the toxic pollutants such as nitro-aromatics, benzene, toluene, phenol, heavy metals etc. with intense colour. The present study focus...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2020.128739
更新日期:2020-10-26 00:00:00
abstract::Photochemical behavior of various polycyclic aromatic hydrocarbons (PAHs) on Fe3+-modified montmorillonite was explored to determine their potential kinetics, pathways, and mechanism under visible light. Depending on the type of PAH molecules, the transformation rate follows the order of benzo[a]pyrene ≈ anthracene > ...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2017.06.106
更新日期:2017-10-01 00:00:00
abstract::In soil, chromium can be found in two main valence states: hexavalent Cr(VI) and trivalent Cr(III). In this study, we investigated the impact of Cr on photosynthetic gas exchange, photosystem II (PSII) activity, Cr translocation and accumulation, proline content and alkaloids production, i.e. scopolamine and hyoscyami...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2008.03.018
更新日期:2008-06-01 00:00:00
abstract::In current work, Prussian blue (PB)- and hydroxyapatite (HAp)-embedded micro-adsorbents (PB-HAp-MAs) were rationally fabricated through an easy and flexible custom-made micronozzle system as a novel bifunctional adsorbent. The adsorption performance of the as-prepared samples was conducted based on the removal of cesi...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2020.128266
更新日期:2021-01-01 00:00:00
abstract::The green credentials of ionic liquids (ILs) are being challenged due to the increasing evidence of their toxicity. The hormetic effects further raised their ecological concern. However, it remained poorly studied on the time-dependent changes of the hormetic effects and the mechanisms. In this study, we investigated ...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2012.11.070
更新日期:2013-04-01 00:00:00
abstract::In southern China revegetation and ecological restoration of many abandoned Mn tailings has become a major concern. To determine the major constraints for plant establishment and evaluate the feasibility of remediation, a comparative study was conducted on Mn tailings and rhizosphere soils at the boundary of the taili...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2008.05.001
更新日期:2008-07-01 00:00:00
abstract::This paper presents results of investigations on the influence of humic substances (humate, HS) on the biological treatment of wastewater containing heavy metals (Cr,Cu,Fe,Mn,Ni, and Zn). Respirometric studies indicated that the investigated system complied with the Haldane model for inhibitory wastes. Chemical analys...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2009.07.036
更新日期:2009-09-01 00:00:00
abstract::To evaluate the body burdens of heavy metals correlated with health impact on school-age children living around a waste incinerator. A total of 81 children from the exposure area and 95 from the control area were recruited in our study. We measured the blood levels of chromium (Cr), cadmium (Cd) and lead (Pb) by an in...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2019.05.016
更新日期:2019-08-01 00:00:00
abstract::Human intervention in the global phosphorus cycle has mobilised nearly half a billion tonnes of the element from phosphate rock into the hydrosphere over the past half century. The resultant water pollution concerns have been the main driver for sustainable phosphorus use (including phosphorus recovery). However the e...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2011.02.032
更新日期:2011-08-01 00:00:00
abstract::Ground discarded tires adsorb naphthalene, toluene, and mercury ions (Hg2+) from aqueous solutions. Their sorption properties and kinetics were determined by batch equilibration techniques at 20 degrees C. The isotherms were linear for naphthalene and toluene and their sorption coefficients were about 1340 and 255 (ml...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/s0045-6535(00)00016-3
更新日期:2000-10-01 00:00:00
abstract::Lemongrass is a commercially important perennial herb with medicinal value and ability to tolerate high alkaline and saline conditions. Essential oil bearing plants can grow safely in soil contaminated with heavy metals without severe effects on morphology and oil yield. The present study was aimed to assess the essen...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2017.02.065
更新日期:2017-05-01 00:00:00
abstract::We investigated whether polychlorinated biphenyls (PCBs) and water could be simultaneously removed from river sediment by solvent extraction using liquefied dimethyl ether (DME) as the extractant. DME exists in a gaseous state at normal temperature and pressure and can dissolve organic substances and some amount of wa...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2009.12.017
更新日期:2010-02-01 00:00:00
abstract::The biotransformation and mineralization of a mixture of two polycyclic aromatic hydrocarbons (PAHs), anthracene and pyrene, which are known contaminants of soil and groundwater, by an enrichment culture in the presence or absence of 100 mg l(-1) Tergitol NP-10, a non-ionic surfactant, and at temperatures of 10 degree...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2005.02.061
更新日期:2005-11-01 00:00:00
abstract::Red deer antlers have a number of advantages that make them a unique material for monitoring trace elements. As antlers are shed and regrown every year, results of toxicological investigations can be applied to a particular region and time. We analyzed the content of four toxic (Pb, Cd, Hg, As) and three essential (Cu...
journal_title:Chemosphere
pub_type: 历史文章,杂志文章
doi:10.1016/j.chemosphere.2020.128055
更新日期:2020-12-01 00:00:00
abstract::Untreated pharmaceutical pollution and their possibly toxic metabolites, resulting from overloaded wastewater treatment processes, end up in aquatic environments and are hazardous to the ecosystem homeostasis. Biological wastewater remediation could supplement traditional methods and overcome the release of these biol...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2020.128117
更新日期:2021-01-01 00:00:00
abstract::An experimental study was conducted to investigate the trophic transfer of 137Cs in marine and freshwater food chains, focusing on phytoplankton, zooplankton, and planktivorous fish. Algal concentration factors were 278 in freshwater and 69 in seawater. The weight-normalized uptake rate constants of 137Cs were similar...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2018.06.124
更新日期:2018-10-01 00:00:00
abstract::This work investigates the effect of multifunctional poly (N-isopropyl acrylamide/acrylic acid/N-tert-butylacrylamide) [p(NIPAM-AA-NTBA)] ternary polymer on the sedimentation of kaolin clay - a major fraction of oil sands tailings. A series of linear, uncross-linked p(NIPAM), p(NIPAM/AA), and p(NIPAM/AA/NTBM) were syn...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2017.12.009
更新日期:2018-03-01 00:00:00
abstract::This research investigates the environmental behavior of two widely prescribed cholesterol-lowering statin drugs that are expected to be present at significant concentrations in wastewater influents, namely: atorvastatin and simvastatin. Batch biodegradation experiments suggest that both statins are well degraded duri...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2012.03.066
更新日期:2012-08-01 00:00:00
abstract::Lignin peroxidase (LiP) is excreted by certain lignin-degrading fungi, such as white rot fungus Phanerochaete chrysosporium, in natural environments and is thus widely present in the natural environment. We have found in our earlier studies that LiP mediates effective reactions of a few natural and synthetic estrogens...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2010.03.054
更新日期:2010-06-01 00:00:00
abstract::Pentachlorophenol (PCP) contamination is a severe environmental problem due to its widespread occurrence, toxicity and recalcitrance. In order to gain a better understanding of the fate of PCP in soils, the role of the soil organic matter (SOM) and clay minerals in the PCP sorption-desorption was studied on two bulk f...
journal_title:Chemosphere
pub_type: 杂志文章
doi:10.1016/j.chemosphere.2006.01.017
更新日期:2006-08-01 00:00:00