Abstract:
:Iron nanoparticles (Fe NPs) were synthesized herein through a simple and eco-friendly method using FeCl3 and aqueous plant extract (dimocarpus longan, DL). Compared with Fe NPs prepared via traditional chemical methods, this biogenetic DL-Fe NPs demonstrates higher catalytic activity in Fenton-like reaction to degrade methyl orange (MO) in a wide pH range. It's worth noting that the DL-Fe NPs manifest a superior stability even after storage for at least 28 days. Systematic characterizations indicate that the active biomolecules from plant extract significantly contribute to the superior performance of DL-Fe NPs, by facilitating the dye molecules to be adsorbed on the surfaces of DL-Fe NPs, and providing a stable acid environment for the Fenton-like catalytic reaction. The kinetics study demonstrates this removal process conforms to the pseudo first-order model with the reaction activation energy of 41.6 kJ/mol. Moreover, various typical dyes including congo red, malachite green, methylene blue, eosin-Y and rhodamine B can be dramatically degraded by this DL-Fe NPs with a satisfactory removal efficiency.
journal_name
Chemospherejournal_title
Chemosphereauthors
Yuan M,Fu X,Yu J,Xu Y,Huang J,Li Q,Sun Ddoi
10.1016/j.chemosphere.2020.127618subject
Has Abstractpub_date
2020-12-01 00:00:00pages
127618eissn
0045-6535issn
1879-1298pii
S0045-6535(20)31813-0journal_volume
261pub_type
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