当前位置： SCI文献检索 > ENVIRONMENTAL MONITORING AND ASSESSMENT期刊下所有文献 > Spatial patterns and ratios of ¹³⁷Cs, ⁹⁰Sr, and Pu isotopes in the top layer of undisturbed meadow soils as indicators for contamination origin.

Spatial patterns and ratios of ¹³⁷Cs, ⁹⁰Sr, and Pu isotopes in the top layer of undisturbed meadow soils as indicators for contamination origin.

Abstract：

:Spatial distribution of activity concentrations of (137)Cs, (90)Sr, and (239,240)Pu in the top layer of undisturbed meadow soils was compared between two regional transects across Lithuania: one in the SW region, more affected by the Chernobyl radioactive fallout, and the other in the NE region. Radiochemical, γ-, α-, β-, and mass spectrometric methods were used to determine the radionuclide activity. Our results validate that higher activity concentrations in the top soil layer were present in the SW region, despite the fact that sampling was performed after 22 years of the Chernobyl Nuclear Power Plant (NPP) accident. Using the activity concentration ratio (137)Cs/(239,240)Puglobal, the contribution of the Chernobyl NPP accident to the total radiocesium activity concentrations in these meadow soils was evaluated and found to be in the range of 6.5-59.1%. Meanwhile, the activity concentration ratio (238)Pu/(239,240)Pu showed that Chernobyl-derived Pu occurred at almost half of the sampling sites. The locations with maximal values of 47% of Chernobyl-derived Pu material were close to northeastern Poland, where deposition of most of non-volatile radioisotopes from the Chernobyl plume was determined.

journal_name

Environ Monit Assess

journal_title

Environmental monitoring and assessment

authors

Lukšienė B,Puzas A,Remeikis V,Druteikienė R,Gudelis A,Gvozdaitė R,Buivydas Š,Davidonis R,Kandrotas G

doi

10.1007/s10661-015-4491-9

subject

Has Abstract

pub_date

2015-05-01 00:00:00

pages

268

issue

5

eissn

0167-6369

issn

1573-2959

journal_volume

187

pub_type

杂志文章

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