One-step synthesis of cake-like biosorbents from plant biomass for the effective removal and recovery heavy metals: Effect of plant species and roles of xanthation.

Abstract:

:The continuous production of plant wastes and heavy metal pollution of waters have become widespread unavoidable challenges. Reutilization of plant wastes to treat toxic metal-contaminated water is an eco-friendly way to simultaneously solve these problems. Herein, three cake-like biosorbents were synthesized from tea waste, trimmed lawn grass and Nephrolepis cordifolia leaves through a one-step xanthation modification method combined with lyophilization, respectively. The plant species affected the appearance, structure and mechanical strength of the biosorbents due to the different contents of hydrocarbons and inorganic substances, which influenced the gel-like degree and thus the ability of the particles to pack between water molecules. The maximum adsorption capacities of the modified materials for Pb(II), Cu(II) and Cd(II) were 247.20, 85.80 and 265.31 mg/g, respectively, far higher than those of the original wastes, and the adsorption was selective. These results were mainly attributed to newly introduced -(CS)-S-Na groups, which triggered ion exchange, complexation and microprecipitation between heavy metal ions and functional groups. As-prepared biosorbents owned an excellent regenerability, which contributed to recovery heavy metals. The physicochemical properties and adsorption performances of the modified materials indicated that xanthation is a universal modification method suited to different plant biomasses with great potential to purify heavy metal-contaminated water. These biosorbents with excellent separability and regenerability might be promising for continuous-flow sewage treatment.

journal_name

Chemosphere

journal_title

Chemosphere

authors

Wang N,Qiu Y,Hu K,Huang C,Xiang J,Li H,Tang J,Wang J,Xiao T

doi

10.1016/j.chemosphere.2020.129129

subject

Has Abstract

pub_date

2021-03-01 00:00:00

pages

129129

eissn

0045-6535

issn

1879-1298

pii

S0045-6535(20)33326-9

journal_volume

266

pub_type

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