A tied Fermi liquid to Luttinger liquid model for nonlinear transport in conducting polymers.

Abstract:

:Organic conjugated polymers demonstrate great potential in transistors, solar cells and light-emitting diodes, whose performances are fundamentally governed by charge transport. However, the morphology-property relationships and the underpinning charge transport mechanisms remain unclear. Particularly, whether the nonlinear charge transport in conducting polymers is appropriately formulated within non-Fermi liquids is not clear. In this work, via varying crystalline degrees of samples, we carry out systematic investigations on the charge transport nonlinearity in conducting polymers. Possible charge carriers' dimensionality is discussed when varying the molecular chain's crystalline orders. A heterogeneous-resistive-network (HRN) model is proposed based on the tied-link between Fermi liquids (FL) and Luttinger liquids (LL), related to the high-ordered crystalline zones and weak-coupled amorphous regions, respectively. The HRN model is supported by precise electrical and microstructural characterizations, together with theoretic evaluations, which well describes the nonlinear transport behaviors and provides new insights into the microstructure-correlated charge transport in organic solids.

journal_name

Nat Commun

journal_title

Nature communications

authors

Wang J,Niu J,Shao B,Yang G,Lu C,Li M,Zhou Z,Chuai X,Chen J,Lu N,Huang B,Wang Y,Li L,Liu M

doi

10.1038/s41467-020-20238-5

subject

Has Abstract

pub_date

2021-01-04 00:00:00

pages

58

issue

1

issn

2041-1723

pii

10.1038/s41467-020-20238-5

journal_volume

12

pub_type

杂志文章
  • Crystal structures of ryanodine receptor SPRY1 and tandem-repeat domains reveal a critical FKBP12 binding determinant.

    abstract::Ryanodine receptors (RyRs) form calcium release channels located in the membranes of the sarcoplasmic and endoplasmic reticulum. RyRs play a major role in excitation-contraction coupling and other Ca(2+)-dependent signalling events, and consist of several globular domains that together form a large assembly. Here we d...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms8947

    authors: Yuchi Z,Yuen SM,Lau K,Underhill AQ,Cornea RL,Fessenden JD,Van Petegem F

    更新日期:2015-08-06 00:00:00

  • Interfacial control of oxygen vacancy doping and electrical conduction in thin film oxide heterostructures.

    abstract::Oxygen vacancies in proximity to surfaces and heterointerfaces in oxide thin film heterostructures have major effects on properties, resulting, for example, in emergent conduction behaviour, large changes in metal-insulator transition temperatures or enhanced catalytic activity. Here we report the discovery of a means...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms11892

    authors: Veal BW,Kim SK,Zapol P,Iddir H,Baldo PM,Eastman JA

    更新日期:2016-06-10 00:00:00

  • Exosomes harbor B cell targets in pancreatic adenocarcinoma and exert decoy function against complement-mediated cytotoxicity.

    abstract::Although B cell response is frequently found in cancer, there is little evidence that it alters tumor development or progression. The process through which tumor-associated antigens trigger humoral response is not well delineated. We investigate the repertoire of antigens associated with humoral immune response in pan...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-08109-6

    authors: Capello M,Vykoukal JV,Katayama H,Bantis LE,Wang H,Kundnani DL,Aguilar-Bonavides C,Aguilar M,Tripathi SC,Dhillon DS,Momin AA,Peters H,Katz MH,Alvarez H,Bernard V,Ferri-Borgogno S,Brand R,Adler DG,Firpo MA,Mulvihill S

    更新日期:2019-01-16 00:00:00

  • Arrays of giant octagonal and square cylinders by liquid crystalline self-assembly of X-shaped polyphilic molecules.

    abstract::Nanopatterning by molecular self-assembly has been a topic of intense research in pursuit of 'bottom-up' methods of generating structures for use in nanotechnology. The systems most widely studied have been two- and three-dimensional morphologies of block copolymers. However, T- and X-shaped polyphilic liquid crystals...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms2096

    authors: Liu F,Kieffer R,Zeng X,Pelz K,Prehm M,Ungar G,Tschierske C

    更新日期:2012-01-01 00:00:00

  • A diverse intrinsic antibiotic resistome from a cave bacterium.

    abstract::Antibiotic resistance is ancient and widespread in environmental bacteria. These are therefore reservoirs of resistance elements and reflective of the natural history of antibiotics and resistance. In a previous study, we discovered that multi-drug resistance is common in bacteria isolated from Lechuguilla Cave, an un...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms13803

    authors: Pawlowski AC,Wang W,Koteva K,Barton HA,McArthur AG,Wright GD

    更新日期:2016-12-08 00:00:00

  • IL-6 receptor blockade corrects defects of XIAP-deficient regulatory T cells.

    abstract::X-linked lymphoproliferative syndrome type-2 (XLP-2) is a primary immunodeficiency disease attributed to XIAP mutation and is triggered by infection. Here, we show that mouse Xiap-/- regulatory T (Treg) cells and human XIAP-deficient Treg cells are defective in suppressive function. The Xiap-/- Treg cell defect is lin...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-02862-4

    authors: Hsieh WC,Hsu TS,Chang YJ,Lai MZ

    更新日期:2018-01-31 00:00:00

  • The anti-sigma factor RsrA responds to oxidative stress by reburying its hydrophobic core.

    abstract::Redox-regulated effector systems that counteract oxidative stress are essential for all forms of life. Here we uncover a new paradigm for sensing oxidative stress centred on the hydrophobic core of a sensor protein. RsrA is an archetypal zinc-binding anti-sigma factor that responds to disulfide stress in the cytoplasm...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms12194

    authors: Rajasekar KV,Zdanowski K,Yan J,Hopper JT,Francis ML,Seepersad C,Sharp C,Pecqueur L,Werner JM,Robinson CV,Mohammed S,Potts JR,Kleanthous C

    更新日期:2016-07-19 00:00:00

  • A generalized non-local optical response theory for plasmonic nanostructures.

    abstract::Metallic nanostructures exhibit a multitude of optical resonances associated with localized surface plasmon excitations. Recent observations of plasmonic phenomena at the sub-nanometre to atomic scale have stimulated the development of various sophisticated theoretical approaches for their description. Here instead we...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms4809

    authors: Mortensen NA,Raza S,Wubs M,Søndergaard T,Bozhevolnyi SI

    更新日期:2014-05-02 00:00:00

  • Shared developmental programme strongly constrains beak shape diversity in songbirds.

    abstract::The striking diversity of bird beak shapes is an outcome of natural selection, yet the relative importance of the limitations imposed by the process of beak development on generating such variation is unclear. Untangling these factors requires mapping developmental mechanisms over a phylogeny far exceeding model syste...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms4700

    authors: Fritz JA,Brancale J,Tokita M,Burns KJ,Hawkins MB,Abzhanov A,Brenner MP

    更新日期:2014-04-16 00:00:00

  • Regulation of PCNA cycling on replicating DNA by RFC and RFC-like complexes.

    abstract::Replication-Factor-C (RFC) and RFC-like complexes (RLCs) mediate chromatin engagement of the proliferating cell nuclear antigen (PCNA). It remains controversial how RFC and RLCs cooperate to regulate PCNA loading and unloading. Here, we show the distinct PCNA loading or unloading activity of each clamp loader. ATAD5-R...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-10376-w

    authors: Kang MS,Ryu E,Lee SW,Park J,Ha NY,Ra JS,Kim YJ,Kim J,Abdel-Rahman M,Park SH,Lee KY,Kim H,Kang S,Myung K

    更新日期:2019-06-03 00:00:00

  • Author Correction: Fermiology and electron dynamics of trilayer nickelate La4Ni3O10.

    abstract::The original version of this Article contained errors in Fig. 2, Fig. 3a-c and Supplementary Fig. 2. In Fig. 2g and Supplementary Fig. 2, the band structure plot calculated from density function theory (DFT) had a missing band of mainly z2 character that starts at about - 0.25 eV at the Y point and disperses downwards...

    journal_title:Nature communications

    pub_type: 杂志文章,已发布勘误

    doi:10.1038/s41467-018-04105-y

    authors: Li H,Zhou X,Nummy T,Zhang J,Pardo V,Pickett WE,Mitchell JF,Dessau DS

    更新日期:2018-05-11 00:00:00

  • Author Correction: GWAS for male-pattern baldness identifies 71 susceptibility loci explaining 38% of the risk.

    abstract::We have been alerted that in our recent Article the calculations used to transform the heritability from the observed scale to the liability scale did not take into account the individuals in category 2 of the baldness scale, who were removed in our original analysis. This led to an overestimation of the heritability ...

    journal_title:Nature communications

    pub_type: 杂志文章,已发布勘误

    doi:10.1038/s41467-018-04857-7

    authors: Pirastu N,Joshi PK,de Vries PS,Cornelis MC,McKeigue PM,Keum N,Franceschini N,Colombo M,Giovannucci EL,Spiliopoulou A,Franke L,North KE,Kraft P,Morrison AC,Esko T,Wilson JF

    更新日期:2018-06-29 00:00:00

  • Quantitative bounds on morphodynamics and implications for reading the sedimentary record.

    abstract::Sedimentary rocks are the archives of environmental conditions and ancient planetary surface processes that led to their formation. Reconstructions of Earth's past surface behaviour from the physical sedimentary record remain controversial, however, in part because we lack a quantitative framework to deconvolve intern...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms4298

    authors: Ganti V,Lamb MP,McElroy B

    更新日期:2014-02-28 00:00:00

  • Single spin localization and manipulation in graphene open-shell nanostructures.

    abstract::Turning graphene magnetic is a promising challenge to make it an active material for spintronics. Predictions state that graphene structures with specific shapes can spontaneously develop magnetism driven by Coulomb repulsion of π-electrons, but its experimental verification is demanding. Here, we report on the observ...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-08060-6

    authors: Li J,Sanz S,Corso M,Choi DJ,Peña D,Frederiksen T,Pascual JI

    更新日期:2019-01-14 00:00:00

  • Integrative transcriptome imputation reveals tissue-specific and shared biological mechanisms mediating susceptibility to complex traits.

    abstract::Transcriptome-wide association studies integrate gene expression data with common risk variation to identify gene-trait associations. By incorporating epigenome data to estimate the functional importance of genetic variation on gene expression, we generate a small but significant improvement in the accuracy of transcr...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-019-11874-7

    authors: Zhang W,Voloudakis G,Rajagopal VM,Readhead B,Dudley JT,Schadt EE,Björkegren JLM,Kim Y,Fullard JF,Hoffman GE,Roussos P

    更新日期:2019-08-23 00:00:00

  • Enthalpy-entropy compensation of atomic diffusion originates from softening of low frequency phonons.

    abstract::Experimental data accumulated over more than 120 years show not only that diffusion coefficients of impurities ordinarily obey the Arrhenius law in crystalline solids, but also that diffusion pre-exponential factors measured in a same solid increase exponentially with activation energies. This so-called compensation e...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-17812-2

    authors: Gelin S,Champagne-Ruel A,Mousseau N

    更新日期:2020-08-07 00:00:00

  • Relativistic and resonant effects in the ionization of heavy atoms by ultra-intense hard X-rays.

    abstract::An accurate description of the interaction of intense hard X-ray pulses with heavy atoms, which is crucial for many applications of free-electron lasers, represents a hitherto unresolved challenge for theory because of the enormous number of electronic configurations and relativistic effects, which need to be taken in...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-06745-6

    authors: Rudek B,Toyota K,Foucar L,Erk B,Boll R,Bomme C,Correa J,Carron S,Boutet S,Williams GJ,Ferguson KR,Alonso-Mori R,Koglin JE,Gorkhover T,Bucher M,Lehmann CS,Krässig B,Southworth SH,Young L,Bostedt C,Ueda K,Marchenk

    更新日期:2018-10-10 00:00:00

  • Genetic architecture of epigenetic and neuronal ageing rates in human brain regions.

    abstract::Identifying genes regulating the pace of epigenetic ageing represents a new frontier in genome-wide association studies (GWASs). Here using 1,796 brain samples from 1,163 individuals, we carry out a GWAS of two DNA methylation-based biomarkers of brain age: the epigenetic ageing rate and estimated proportion of neuron...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms15353

    authors: Lu AT,Hannon E,Levine ME,Crimmins EM,Lunnon K,Mill J,Geschwind DH,Horvath S

    更新日期:2017-05-18 00:00:00

  • ABL1 regulates spindle orientation in adherent cells and mammalian skin.

    abstract::Despite the growing evidence for the regulated spindle orientation in mammals, a systematic approach for identifying the responsible genes in mammalian cells has not been established. Here we perform a kinase-targeting RNAi screen in HeLa cells and identify ABL1 as a novel regulator of spindle orientation. Knockdown o...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms1634

    authors: Matsumura S,Hamasaki M,Yamamoto T,Ebisuya M,Sato M,Nishida E,Toyoshima F

    更新日期:2012-01-17 00:00:00

  • Endocrine disruptors induce perturbations in endoplasmic reticulum and mitochondria of human pluripotent stem cell derivatives.

    abstract::Persistent exposure to man-made endocrine disrupting chemicals during fetal endocrine development may lead to disruption of metabolic homeostasis contributing to childhood obesity. Limited cellular platforms exist to test endocrine disrupting chemical-induced developmental abnormalities in human endocrine tissues. Her...

    journal_title:Nature communications

    pub_type: 杂志文章,收录出版

    doi:10.1038/s41467-017-00254-8

    authors: Rajamani U,Gross AR,Ocampo C,Andres AM,Gottlieb RA,Sareen D

    更新日期:2017-08-09 00:00:00

  • JAM-A regulates cortical dynein localization through Cdc42 to control planar spindle orientation during mitosis.

    abstract::Planar spindle orientation in polarized epithelial cells depends on the precise localization of the dynein-dynactin motor protein complex at the lateral cortex. The contribution of cell adhesion molecules to the cortical localization of the dynein-dynactin complex is poorly understood. Here we find that junctional adh...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms9128

    authors: Tuncay H,Brinkmann BF,Steinbacher T,Schürmann A,Gerke V,Iden S,Ebnet K

    更新日期:2015-08-26 00:00:00

  • Bacterial coinfection restrains antiviral CD8 T-cell response via LPS-induced inhibitory NK cells.

    abstract::Infection of specific pathogen-free mice with lymphocytic choriomeningitis virus (LCMV) is a widely used model to study antiviral T-cell immunity. Infections in the real world, however, are often accompanied by coinfections with unrelated pathogens. Here we show that in mice, systemic coinfection with E. coli suppress...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-06609-z

    authors: Straub T,Freudenberg MA,Schleicher U,Bogdan C,Gasteiger G,Pircher H

    更新日期:2018-10-08 00:00:00

  • HIV envelope V3 region mimic embodies key features of a broadly neutralizing antibody lineage epitope.

    abstract::HIV-1 envelope (Env) mimetics are candidate components of prophylactic vaccines and potential therapeutics. Here we use a synthetic V3-glycopeptide ("Man9-V3") for structural studies of an HIV Env third variable loop (V3)-glycan directed, broadly neutralizing antibody (bnAb) lineage ("DH270"), to visualize the epitope...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-018-03565-6

    authors: Fera D,Lee MS,Wiehe K,Meyerhoff RR,Piai A,Bonsignori M,Aussedat B,Walkowicz WE,Ton T,Zhou JO,Danishefsky S,Haynes BF,Harrison SC

    更新日期:2018-03-16 00:00:00

  • Solvent-driven electron trapping and mass transport in reduced graphites to access perfect graphene.

    abstract::Herein, we report on a significant discovery, namely, the quantitative discharging of reduced graphite forms, such as graphite intercalation compounds, graphenide dispersions and graphenides deposited on surfaces with the simple solvent benzonitrile. Because of its comparatively low reduction potential, benzonitrile i...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms12411

    authors: Vecera P,Holzwarth J,Edelthalhammer KF,Mundloch U,Peterlik H,Hauke F,Hirsch A

    更新日期:2016-08-10 00:00:00

  • Efficient and tuneable photoluminescent boehmite hybrid nanoplates lacking metal activator centres for single-phase white LEDs.

    abstract::White light-emitting diodes (WLEDs) are candidates to revolutionize the lighting industry towards energy efficient and environmental friendly lighting and displays. The current challenges in WLEDs encompass high luminous efficiency, chromatic stability, high colour-rending index and price competitiveness. Recently, th...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms6702

    authors: Bai X,Caputo G,Hao Z,Freitas VT,Zhang J,Longo RL,Malta OL,Ferreira RA,Pinna N

    更新日期:2014-12-08 00:00:00

  • Geologically-inspired strong bulk ceramics made with water at room temperature.

    abstract::Dense ceramic materials can form in nature under mild temperatures in water. By contrast, man-made ceramics often require sintering temperatures in excess of 1,400 °C for densification. Chemical strategies inspired by biomineralization processes have been demonstrated but remain limited to the fabrication of thin film...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms14655

    authors: Bouville F,Studart AR

    更新日期:2017-03-06 00:00:00

  • A quantum spin-probe molecular microscope.

    abstract::Imaging the atomic structure of a single biomolecule is an important challenge in the physical biosciences. Whilst existing techniques all rely on averaging over large ensembles of molecules, the single-molecule realm remains unsolved. Here we present a protocol for 3D magnetic resonance imaging of a single molecule u...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms12667

    authors: Perunicic VS,Hill CD,Hall LT,Hollenberg LC

    更新日期:2016-10-11 00:00:00

  • Formation of nitrogen-doped graphene nanoscrolls by adsorption of magnetic γ-Fe2O3 nanoparticles.

    abstract::Graphene nanoscrolls are Archimedean-type spirals formed by rolling single-layer graphene sheets. Their unique structure makes them conceptually interesting and understanding their formation gives important information on the manipulation and characteristics of various carbon nanostructures. Here we report a 100% effi...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms3319

    authors: Sharifi T,Gracia-Espino E,Barzegar HR,Jia X,Nitze F,Hu G,Nordblad P,Tai CW,Wågberg T

    更新日期:2013-01-01 00:00:00

  • eIF6 coordinates insulin sensitivity and lipid metabolism by coupling translation to transcription.

    abstract::Insulin regulates glycaemia, lipogenesis and increases mRNA translation. Cells with reduced eukaryotic initiation factor 6 (eIF6) do not increase translation in response to insulin. The role of insulin-regulated translation is unknown. Here we show that reduction of insulin-regulated translation in mice heterozygous f...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/ncomms9261

    authors: Brina D,Miluzio A,Ricciardi S,Clarke K,Davidsen PK,Viero G,Tebaldi T,Offenhäuser N,Rozman J,Rathkolb B,Neschen S,Klingenspor M,Wolf E,Gailus-Durner V,Fuchs H,Hrabe de Angelis M,Quattrone A,Falciani F,Biffo S

    更新日期:2015-09-18 00:00:00

  • Origin of micro-scale heterogeneity in polymerisation of photo-activated resin composites.

    abstract::Photo-activated resin composites are widely used in industry and medicine. Despite extensive chemical characterisation, the micro-scale pattern of resin matrix reactive group conversion between filler particles is not fully understood. Using an advanced synchrotron-based wide-field IR imaging system and state-of-the-a...

    journal_title:Nature communications

    pub_type: 杂志文章

    doi:10.1038/s41467-020-15669-z

    authors: Sirovica S,Solheim JH,Skoda MWA,Hirschmugl CJ,Mattson EC,Aboualizadeh E,Guo Y,Chen X,Kohler A,Romanyk DL,Rosendahl SM,Morsch S,Martin RA,Addison O

    更新日期:2020-04-15 00:00:00