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Flexible thermoelectric films formed using integrated nanocomposites with single-wall carbon nanotubes and Bi2Te3 nanoplates via solvothermal synthesis.

Abstract：

:Single-wall carbon nanotubes (SWCNTs) and Bi2Te3 nanoplates are very promising thermoelectric materials for energy harvesting. When these two materials are combined, the resulting nanocomposites exhibit high thermoelectric performance and excellent flexibility. However, simple mixing of these materials is not effective in realizing high performance. Therefore, we fabricated integrated nanocomposites by adding SWCNTs during solvothermal synthesis for the crystallization of Bi2Te3 nanoplates and prepared flexible integrated nanocomposite films by drop-casting. The integrated nanocomposite films exhibited high electrical conductivity and an n-type Seebeck coefficient owing to the low contact resistance between the nanoplates and SWCNTs. The maximum power factor was 1.38 μW/(cm K2), which was 23 times higher than that of a simple nanocomposite film formed by mixing SWCNTs during drop-casting, but excluding solvothermal synthesis. Moreover, the integrated nanocomposite films maintained their thermoelectric properties through 500 bending cycles.

journal_name

Sci Rep

journal_title

Scientific reports

authors

Yabuki H,Yonezawa S,Eguchi R,Takashiri M

doi

10.1038/s41598-020-73808-4

subject

Has Abstract

pub_date

2020-10-12 00:00:00

pages

17031

issue

1

issn

2045-2322

pii

10.1038/s41598-020-73808-4

journal_volume

10

pub_type

杂志文章

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